ELECTRON-SCATTERING FROM HE-4 AND NE CLUSTERS - DETERMINATION OF THE CLUSTER DENSITY FROM THE ELECTRONIC SURFACE-BARRIER POTENTIAL

被引:53
作者
MARTINI, K
TOENNIES, JP
WINKLER, C
机构
[1] UNIV MASSACHUSETTS,DEPT PHYS,AMHERST,MA 01002
[2] LEOPOLD FRANZENS UNIV,INST IONENPHYS,A-6020 INNSBRUCK,AUSTRIA
关键词
D O I
10.1016/0009-2614(91)90277-G
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A monoenergetic beam of electrons is scattered from a beam of He-4 clusters. The angular distribution of the scattered electronically excited atoms and clusters is measured by an open Venetian-blind multiplier, which is rotatable in the plane of both beams. The threshold electron energy for excitation of the clusters shows a shift to higher energies with respect to the atom component by between 0.6 and 1.1 eV depending on the cluster source temperature T0 (P0 = 20 bar in all experiments). The observed potential shift E(b) is attributed to the surface barrier for penetration of the electrons into the cluster. From the known dependence of E(b) on density the core densities of the helium clusters is estimated to vary between n = 1.2 x 10(22) cm-3 and n = 2.2 x 10(22) cm-3 for T0 = 14.9 and 11 K, respectively. The latter values agree with those for bulk liquid helium. For Ne clusters, E(b) = 0.7 +/- 0.3 eV independent of the source conditions.
引用
收藏
页码:429 / 434
页数:6
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