PHOTOELECTRONS FROM NEGATIVE DIMERS AND CLUSTERS OF SULFUR-DIOXIDE

被引:12
作者
DRESCH, T
KRAMER, H
THURNER, Y
WEBER, R
机构
[1] Fakultät für Physik, Universität Konstanz
关键词
D O I
10.1016/0009-2614(91)85070-D
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Photoelectrons originating from sulfur dioxide cluster anions were studied using a tandem mass spectrometer combined with an electron detector and intracavity argon-ion and dye lasers. The absolute photodetachment cross section of the dimer anion increases to (8 +/- 1) x 10(-19) cm2 at 2.71 eV photon energy. Electrons detected from the interaction of photons with sulfur dioxide clusters were found to be produced in sequential two-step processes only, revealing a lower bound of the cluster's detachment threshold energy of 2.7 eV.
引用
收藏
页码:383 / 388
页数:6
相关论文
共 20 条
[1]  
[Anonymous], 1973, MOBILITY DIFFUSION I
[2]   ELECTRON-ATTACHMENT TO MOLECULAR CLUSTERS BY COLLISIONAL CHARGE-TRANSFER [J].
BOWEN, KH ;
LIESEGANG, GW ;
SANDERS, RA ;
HERSCHBACH, DR .
JOURNAL OF PHYSICAL CHEMISTRY, 1983, 87 (04) :557-565
[3]   OXYGEN METASTABLE ATOM PRODUCTION THROUGH PHOTODETACHMENT [J].
BRANSCOMB, LM ;
SMITH, SJ ;
TISONE, G .
JOURNAL OF CHEMICAL PHYSICS, 1965, 43 (08) :2906-+
[4]   THE USE OF SIMILARITY PROFILES IN STUDYING CLUSTER FORMATION IN MOLECULAR-BEAMS - EVIDENCE FOR THE ROLE OF PRE-EXISTING DIMERS [J].
BREEN, JJ ;
KILGORE, K ;
STEPHAN, K ;
HOFMANNSIEVERT, R ;
KAY, BD ;
KEESEE, RG ;
MARK, TD ;
CASTLEMAN, AW .
CHEMICAL PHYSICS, 1984, 91 (02) :305-313
[5]   LASER PHOTODETACHMENT DETERMINATION OF ELECTRON AFFINITIES OF OH, NH2, NH, SO2, AND S2 [J].
CELOTTA, RJ ;
BENNETT, RA ;
HALL, JL .
JOURNAL OF CHEMICAL PHYSICS, 1974, 60 (05) :1740-1745
[6]  
DRESCH T, IN PRESS
[7]  
Ellis H. B. Jr., 1983, Journal of Chemical Physics, V78, P6541, DOI 10.1063/1.444702
[8]  
FELDMANN D, 1970, Z NATURFORSCH PT A, VA 25, P621
[9]   ULTRAHIGH-RESOLUTION STUDY OF AUTODETACHMENT IN C-2- [J].
HEFTER, U ;
MEAD, RD ;
SCHULZ, PA ;
LINEBERGER, WC .
PHYSICAL REVIEW A, 1983, 28 (03) :1429-1439
[10]   PHOTODESTRUCTION OF IONS CONTAINING SULFUR-DIOXIDE [J].
HODGES, RV ;
VANDERHOFF, JA .
JOURNAL OF CHEMICAL PHYSICS, 1980, 72 (06) :3517-3521