CARBON-DIOXIDE REFORMING OF METHANE ON SUPPORTED NICKEL-CATALYSTS

被引:57
作者
TAKANO, A
TAGAWA, T
GOTO, S
机构
[1] Department of Chemical Engineering, Nagoya University
关键词
CHEMICAL REACTION; CATALYST; CARBON DIOXIDE; METHANE; KINETICS; CARBON DIOXIDE REFORMING; STEAM REFORMING;
D O I
10.1252/jcej.27.727
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
The reforming of CH4 with CO2 using various Ni catalysts has been investigated. As a result of screening tests, the selection of supports was found to be very important to control the catalytic activity of Ni. Among the various supports, ceramic foam and Al2O3 supports incorporating industrial steam reforming catalysts showed higher activities than SiO2 supports. The kinetic study has shown that the results could be expressed by a simple power-law equation for the three activated catalysts. The effect of the support was also studied. The results showed the importance of the acid-base property of the catalyst.
引用
收藏
页码:727 / 731
页数:5
相关论文
共 21 条
[1]   ROLE OF URANIA AND ALUMINA AS SUPPORTS IN STEAM REFORMING OF N-BUTANE AT PRESSURE OVER NICKEL-CONTAINING CATALYSTS [J].
BHATTA, KSM ;
DIXON, GM .
INDUSTRIAL & ENGINEERING CHEMISTRY PRODUCT RESEARCH AND DEVELOPMENT, 1969, 8 (03) :324-&
[2]   ACTIVATION OF CH4 AND ITS REACTION WITH CO2 OVER SUPPORTED RH CATALYSTS [J].
ERDOHELYI, A ;
CSERENYI, J ;
SOLYMOSI, F .
JOURNAL OF CATALYSIS, 1993, 141 (01) :287-299
[3]   SYNTHESIS AND CHARACTERIZATION OF CATALYSTS IN THE SYSTEM AL2O3-MGO-NIO-NI FOR METHANE REFORMING WITH CO2 [J].
GADALLA, AM ;
SOMMER, ME .
JOURNAL OF THE AMERICAN CERAMIC SOCIETY, 1989, 72 (04) :683-687
[4]   THE ROLE OF CATALYST SUPPORT ON THE ACTIVITY OF NICKEL FOR REFORMING METHANE WITH CO2 [J].
GADALLA, AM ;
BOWER, B .
CHEMICAL ENGINEERING SCIENCE, 1988, 43 (11) :3049-3062
[5]  
GADALLA AM, 1989, CHEM ENG SCI, V44, P2825
[6]  
HOUGEN OA, 1960, CHEM PROCESS PRINC 2, P1042
[7]  
KOIDE H, 1993, KAGAKU KOGAKU, V57, P614
[8]  
NAKAMURA J, 1993, SHOKUBAI CATALYST, V35, P478
[9]   HYDROGEN TRANSFER-REACTION BETWEEN ALCOHOLS AND ACETONE [J].
NIIYAMA, H ;
ECHIGOYA, E .
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 1972, 45 (03) :938-+
[10]   ISOMERIZATION OF PROPYLENE-OXIDE ON METAL-OXIDES AND SILICA-MAGNESIA CATALYSTS [J].
OKAMOTO, Y ;
IMANAKA, T ;
TERANISH.S .
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 1973, 46 (01) :4-8