GLOBAL INCREASE OF SF6 OBSERVED IN THE ATMOSPHERE

被引:73
作者
MAISS, M
LEVIN, I
机构
[1] Institut für Umweltphysik, University of Heidelberg
关键词
D O I
10.1029/94GL00179
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
High precision long-term observations of the trace gas sulphur hexafluoride (SF6) in background air at Neumayer station, Antarctica (1986-1991), and at Izana observatory, Tenerife (1991-1992), are presented. Since the very first measurements in 1970 (0.03 pptv), the purely anthropogenic greenhouse gas SF6 has increased by two orders of magnitude to a global mean value of 2.8 pptv in 1992. The observations can best be fitted by a quadratic curve with a recent increase rate of 8.3% yr-1. A significant north-south gradient of 0.29 pptv is observed. From this gradient an interhemispheric exchange time of 1.4 years is derived. A modeled atmospheric budget history agrees reasonably well with estimates of global SF6 production rates and leads to an extrapolated SF6 concentration of about 20 pptv for the year 2030.
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收藏
页码:569 / 572
页数:4
相关论文
共 25 条
[1]   ANALYSIS OF GLOBAL BUDGETS OF HALOCARBONS [J].
CHANG, JS ;
PENNER, JE .
ATMOSPHERIC ENVIRONMENT, 1978, 12 (09) :1867-1873
[2]   MEASUREMENTS OF SOME HALOGENATED COMPOUNDS IN AIR OVER EUROPE [J].
DEBORTOLI, M ;
PECCHIO, E .
ATMOSPHERIC ENVIRONMENT, 1976, 10 (11) :921-923
[3]   ON-SITE MEASUREMENT OF ATMOSPHERIC TRACER GASES [J].
ELIAS, L ;
MCCOOEYE, M ;
GARDNER, G .
GEOPHYSICAL RESEARCH LETTERS, 1976, 3 (01) :17-20
[4]   GAS-CHROMATOGRAPHIC MEASUREMENTS OF ATMOSPHERIC SULFUR-HEXAFLUORIDE [J].
HIROTA, M ;
MURAMATSU, H .
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 1986, 59 (01) :329-331
[5]   ATMOSPHERIC DISTRIBUTION OF KR-85 SIMULATED WITH A GENERAL-CIRCULATION MODEL [J].
JACOB, DJ ;
PRATHER, MJ ;
WOFSY, SC ;
MCELROY, MB .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1987, 92 (D6) :6614-6626
[6]   ATMOSPHERIC SULFUR-HEXAFLUORIDE - SOURCES, SINKS AND GREENHOUSE WARMING [J].
KO, MKW ;
SZE, ND ;
WANG, WC ;
SHIA, G ;
GOLDMAN, A ;
MURCRAY, FJ ;
MURCRAY, DG ;
RINSLAND, CP .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1993, 98 (D6) :10499-10507
[7]   TRENDS IN STRATOSPHERIC CONCENTRATIONS OF TRACE GASES IN THE NORTHERN HEMISPHERE DURING THE YEARS 1974-1979 [J].
LEIFER, R ;
LARSEN, R ;
TOONKEL, L .
GEOPHYSICAL RESEARCH LETTERS, 1982, 9 (07) :755-758
[8]  
LEVIN I, 1992, RADIOCARBON AFTER FOUR DECADES, P503
[9]   ATMOSPHERIC FLUORINE COMPOUNDS AS INDICATORS OF AIR MOVEMENTS [J].
LOVELOCK, JE .
NATURE, 1971, 230 (5293) :379-&
[10]  
MAISS M, 1992, THESIS U HEIDELBERG