SHELL STRUCTURE OF CLUSTERS

被引:166
作者
MARTIN, TP
BERGMANN, T
GOHLICH, H
LANGE, T
机构
[1] Max-Planck-Institut für Festkörperforschung, 7000 Stuttgart 80
关键词
D O I
10.1021/j100170a009
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The properties of bulk metal are so different from those of a metal atom that it is sometimes hard to imagine how they might be related. However, a connection can be established by studying a succession of clusters containing 2, 3, 4, 5, ... atoms. If the properties of the solid were found to evolve gradually and continuously with increasing cluster size, this type of investigation would not really be of much interest. But nature has presented us with a different situation. The properties of clusters change not continuously but often periodically with cluster size. This is due to the formation of shells: shells of electrons and shells of atoms.
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收藏
页码:6421 / 6429
页数:9
相关论文
共 52 条
[1]  
[Anonymous], 1979, ADV CHEM PHYS, DOI DOI 10.1002/9780470142592.CH2
[2]   DISTRIBUTION OF EIGENFREQUENCIES FOR WAVE-EQUATION IN A FINITE DOMAIN .3. EIGENFREQUENCY DENSITY OSCILLATIONS [J].
BALIAN, R ;
BLOCH, C .
ANNALS OF PHYSICS, 1972, 69 (01) :76-&
[3]   ON HYBRIDIZATION AND BONDING IN THE ALKALINE-EARTHS - BE, MG, AND CA [J].
BAUSCHLICHER, CW ;
BAGUS, PS ;
COX, BN .
JOURNAL OF CHEMICAL PHYSICS, 1982, 77 (08) :4032-4038
[4]   SPUTTERED METAL CLUSTER IONS - UNIMOLECULAR DECOMPOSITION AND COLLISION-INDUCED FRAGMENTATION [J].
BEGEMANN, W ;
DREIHOFER, S ;
MEIWESBROER, KH ;
LUTZ, HO .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1986, 3 (2-3) :183-188
[5]   EVIDENCE OF ELECTRONIC SHELL STRUCTURE IN CS-O CLUSTERS [J].
BERGMANN, T ;
LIMBERGER, H ;
MARTIN, TP .
PHYSICAL REVIEW LETTERS, 1988, 60 (17) :1767-1770
[6]   HIGH-RESOLUTION TIME-OF-FLIGHT MASS SPECTROMETERS .2. CROSS BEAM ION OPTICS [J].
BERGMANN, T ;
GOEHLICH, H ;
MARTIN, TP ;
SCHABER, H ;
MALEGIANNAKIS, G .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1990, 61 (10) :2585-2591
[7]   HIGH-RESOLUTION TIME-OF-FLIGHT MASS SPECTROMETERS .2. REFLECTOR DESIGN [J].
BERGMANN, T ;
MARTIN, TP ;
SCHABER, H .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1990, 61 (10) :2592-2600
[8]   OBSERVATION OF ELECTRONIC SHELL STRUCTURE IN LARGE CESIUM OXIDE CLUSTERS [J].
BERGMANN, T ;
MARTIN, TP .
JOURNAL OF CHEMICAL PHYSICS, 1989, 90 (06) :2848-2855
[9]   MEAN-FIELD QUANTIZATION OF SEVERAL HUNDRED ELECTRONS IN SODIUM METAL-CLUSTERS [J].
BJORNHOLM, S ;
BORGGREEN, J ;
ECHT, O ;
HANSEN, K ;
PEDERSEN, J ;
RASMUSSEN, HD .
PHYSICAL REVIEW LETTERS, 1990, 65 (13) :1627-1630
[10]   DEVELOPMENT OF A 1ST-PRINCIPLES MANY-BODY POTENTIAL FOR BERYLLIUM [J].
BLAISTENBAROJAS, E ;
KHANNA, SN .
PHYSICAL REVIEW LETTERS, 1988, 61 (13) :1477-1480