CHARGE-TRANSFER EXCITONS AND CHI(2) OF MOLECULAR MONOLAYERS

被引：13

作者：

DUBOVSKY, O

MUKAMEL, S

机构：

[1] Department of Chemistry, University of Rochester, Rochester

来源：

JOURNAL OF CHEMICAL PHYSICS | 1992年 / 96卷 / 12期

关键词：

D O I：

10.1063/1.462230

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

The second-order nonlinear susceptibility chi(2) is calculated for a monolayer of donor-acceptor substituted molecules, using equations of motion which map the problem onto the dynamics of coupled anharmonic (exciton) oscillators. New exciton resonances, which may change in character from Frenkel through charge transfer to Wannier excitons, are predicted as the intermolecular charge-transfer coupling is turned on.

引用

页码：9201 / 9211

页数：11

共 41 条

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[2]

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[3]

BLOEMBERGEN N, 1978, INDIAN J PURE AP PHY, V16, P151

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