COLLISIONAL ENERGY-DEPENDENCE OF HE CAPTURE BY INTERNALLY EXCITED C-60 ANIONS

被引:31
作者
SPRANG, H
MAHLKOW, A
CAMPBELL, EEB
机构
[1] Max Born Institut für Nichtlineare Optik und Kurzzeitspektroskopie, D-12474 Berlin
关键词
D O I
10.1016/0009-2614(94)00792-6
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The threshold energy for endohedral He@C60 formation under single collision conditions is shown to depend strongly on the internal energy of the fullerence. Under source conditions in which defects in the fullerene cage structure may be expected (high fluence laser desorption, highly excited ions) the threshold energy may be as low as 3 eV. Oscillatory structure is observed in the capture cross sections as a function of collison energy.
引用
收藏
页码:91 / 97
页数:7
相关论文
共 26 条
[1]  
CALDWELL KA, 1991, J AM CHEM SOC, V113, P8519, DOI 10.1021/ja00022a048
[2]   COLLISION ENERGY-DEPENDENCE OF HE AND NE CAPTURE BY C-60(+) [J].
CAMPBELL, EEB ;
EHLICH, R ;
HIELSCHER, A ;
FRAZAO, JMA ;
HERTEL, IV .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1992, 23 (01) :1-2
[3]  
CAMPBELL EEB, 1993, AIP C P, V295, P697
[4]   NE++C60 COLLISIONS - THE DYNAMICS OF CHARGE AND ENERGY-TRANSFER, FRAGMENTATION, AND ENDOHEDRAL COMPLEX-FORMATION [J].
CHRISTIAN, JF ;
WAN, ZM ;
ANDERSON, SL .
JOURNAL OF CHEMICAL PHYSICS, 1993, 99 (05) :3468-3479
[5]   COLLISIONAL DYNAMICS OF C-60 WITH NOBLE-GAS-ATOMS STUDIED BY MOLECULAR-DYNAMICS WITH EMPIRICAL 2-BODY AND 3-BODY FORCES [J].
EHLICH, R ;
CAMPBELL, EEB ;
KNOSPE, O ;
SCHMIDT, R .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1993, 28 (02) :153-161
[6]   ON THE UNIMOLECULAR FRAGMENTATION OF C-60(+) FULLERENE IONS - THE COMPARISON OF MEASURED AND CALCULATED BREAKDOWN PATTERNS [J].
FOLTIN, M ;
LEZIUS, M ;
SCHEIER, P ;
MARK, TD .
JOURNAL OF CHEMICAL PHYSICS, 1993, 98 (12) :9624-9634
[7]   LANTHANUM COMPLEXES OF SPHEROIDAL CARBON SHELLS [J].
HEATH, JR ;
OBRIEN, SC ;
ZHANG, Q ;
LIU, Y ;
CURL, RF ;
KROTO, HW ;
TITTEL, FK ;
SMALLEY, RE .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1985, 107 (25) :7779-7780
[8]   ABINITIO MO CALCULATION ON THE ENERGY BARRIER FOR THE PENETRATION OF A BENZENE-RING BY A HELIUM ATOM - MODEL STUDIES FOR THE FORMATION OF ENDOHEDRAL HE-AT-THE-COST-OF-C60+ - COMPLEXES BY HIGH-ENERGY BIMOLECULAR REACTIONS [J].
HRUSAK, J ;
BOHME, DK ;
WEISKE, T ;
SCHWARZ, H .
CHEMICAL PHYSICS LETTERS, 1992, 193 (1-3) :97-100
[9]   MELTING THE FULLERENES - A MOLECULAR-DYNAMICS STUDY [J].
KIM, SG ;
TOMANEK, D .
PHYSICAL REVIEW LETTERS, 1994, 72 (15) :2418-2421
[10]   HE CAPTURE BY NEGATIVELY CHARGED BUCKMINSTERFULLERENE [J].
KLEISER, R ;
SPRANG, H ;
FURRER, S ;
CAMPBELL, EEB .
ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1993, 28 (02) :89-90