PICOSECOND PHASE CONJUGATE REFLECTIVITY OF GOLD COLLOIDS BY DEGENERATE 4-WAVE MIXING

被引:25
作者
DUTTON, T
VANWONTERGHEM, B
SALTIEL, S
CHESTNOY, NV
RENTZEPIS, PM
SHEN, TP
ROGOVIN, D
机构
[1] UNIV CALIF IRVINE, DEPT CHEM, IRVINE, CA 92717 USA
[2] ROCKWELL INT CORP, THOUSAND OAKS, CA 91360 USA
关键词
D O I
10.1021/j100366a016
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We measure the efficiency and phase of picosecond phase conjugate reflectivity by degenerate four-wave mixing for colloidal gold suspended in water and in glass. Evidence is found for extremely high χ(3) for the gold particles. However, the efficiency has a power dependence which is not increasing quadratically with pump energy. Small-scale lensing effects become significant at high pump energies. Additionally, both the glass-based and the water-based colloids show a visible "permanent" bleaching effect after absorbing only a few pulses of GW/cm2 intensity. © 1990 American Chemical Society.
引用
收藏
页码:1100 / 1105
页数:6
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