ISOTOPICALLY RESOLVED RAMAN-SPECTRA OF C-60

被引:40
作者
GUHA, S
MENENDEZ, J
PAGE, JB
ADAMS, GB
SPENCER, GS
LEHMAN, JP
GIANNOZZI, P
BARONI, S
机构
[1] IST NAZL FIS MAT,SCUOLA NORMALE SUPER & FORUM FIS TEOR,I-56126 PISA,ITALY
[2] SCUOLA INT SUPER STUDI AVANZATI,I-34014 TRIESTE,ITALY
[3] ARIZONA STATE UNIV,DEPT CHEM & BIOCHEM,TEMPE,AZ 85287
关键词
D O I
10.1103/PhysRevLett.72.3359
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We present high-resolution Raman spectra of C60 molecules. The totally symmetric mode near 1470 cm-1 shows a fine structure which is almost exactly isomorphic with the mass spectrum of the molecule. We show that this surprising result can be explained in terms of isotopically induced frequency shifts and the unique iscosahedral symmetry of the molecule. A comparison of predicted and observed isotope shifts provides a stringent test of vibrational theories for C60.
引用
收藏
页码:3359 / 3362
页数:4
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