ANALYSIS OF ASYMMETRIC FRINGE PATTERNS OF 3RD-HARMONIC GENERATION IN A MOLECULAR-CRYSTAL

被引:10
作者
KOBAYASHI, H
KUBODERA, K
机构
[1] NTT Opto-electronics Laboratories, Atsugi, Kanagawa 243-01
关键词
D O I
10.1063/1.348482
中图分类号
O59 [应用物理学];
学科分类号
摘要
The asymmetric Maker fringe pattern of third-harmonic generation in an anisotropic molecular crystal is analyzed to evaluate the third-order optical susceptibility chi(3). Analysis of a diethyl-amino-nitro-stilbene crystal shows that the molecular axes are not oriented parallel to the crystal surface, but are about 45-degrees relative to the surface. The chi(3) value parallel to the orientation of the molecular axis is estimated to be 1.0 X 10(-11) esu, corresponding to about ten times the chi(3) value perpendicular to that axis.
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页码:3807 / 3810
页数:4
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