SYNTHESIS OF ZSM-5 TYPE ZEOLITES WITH AND WITHOUT TEMPLATE AND EVALUATION OF PHYSICOCHEMICAL PROPERTIES AND ANILINE ALKYLATION ACTIVITY

被引:28
作者
NARAYANAN, S [1 ]
SULTANA, A [1 ]
KRISHNA, K [1 ]
MERIAUDEAU, P [1 ]
NACCACHE, C [1 ]
机构
[1] INST RECH CATALYSE,CNRS,F-69626 VILLEURBANNE,FRANCE
关键词
SYNTHESIS OF ZSM-5; TEMPLATE-FREE ZEOLITES; ZEOLITE MORPHOLOGY; ANILINE ALKYLATION; CATALYTIC EVALUATION;
D O I
10.1007/BF00808329
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
ZSM-5 zeolite containing SiO2/Al2O3 = 28 was synthesised by hydrothermal process with and without template. Characterisation of the zeolites was done using XRD, IR, NMR, SEM and BET surface area measurements. Acidity of the zeolites was measured by ammonia adsorption-desorption. Catalytic activity of HZSM-5 zeolites was evaluated by aniline alkylation, cumene dealkylation, alkylation of benzene with ethylene and propylene and isomerisation of m-xylene. Catalytic activity is discussed from the point of view of zeolite acidity and morphology.
引用
收藏
页码:129 / 138
页数:10
相关论文
共 19 条
[1]  
Berak J., 1985, STUD SURF SCI CAT, V24, P47
[2]   USES OF IR SPECTROSCOPY IN IDENTIFYING ZSM ZEOLITE STRUCTURE [J].
COUDURIER, G ;
NACCACHE, C ;
VEDRINE, JC .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1982, (24) :1413-1415
[3]  
DAI FJ, 1986, NEW DEV ZEOLITE SCI
[4]  
GROSE RW, 1981, Patent No. 4257885
[5]   EFFECTS OF SEED MATERIALS ON A ZEOLITE AND ITS PERFORMANCE OF METHANOL CONVERSION [J].
INUI, T ;
MORINAGA, N ;
ISHIHARA, T ;
KANIE, T ;
TAKEGAMI, Y .
JOURNAL OF CATALYSIS, 1983, 79 (01) :176-184
[6]   PROPERTIES OF THE END MEMBERS IN THE PENTASIL-FAMILY OF ZEOLITES - CHARACTERIZATION AS ADSORBENTS [J].
JACOBS, PA ;
BEYER, HK ;
VALYON, J .
ZEOLITES, 1981, 1 (03) :161-168
[7]  
JACOBS PA, 1987, STUD SURF SCI CATAL, V33, P134
[8]   IDENTIFICATION OF ZSM-TYPE AND OTHER 5-RING CONTAINING ZEOLITES BY IR SPECTROSCOPY [J].
JANSEN, JC ;
VANDERGAAG, FJ ;
VANBEKKUM, H .
ZEOLITES, 1984, 4 (04) :369-372
[9]   CRYSTALLIZATION OF ZEOLITE MORDENITE AND ZSM-5 WITHOUT THE AID OF A TEMPLATE [J].
JOSHI, PN ;
SHAIKH, AA ;
CHUMBHALE, VR ;
RAO, BS ;
SHIRALKAR, VP .
JOURNAL OF INCLUSION PHENOMENA AND MOLECULAR RECOGNITION IN CHEMISTRY, 1992, 13 (02) :171-179
[10]   ON THE CRYSTALLIZATION MECHANISM OF ZEOLITE ZSM-5 .2. MNDO CALCULATIONS OF BASIC CHARACTERISTICS OF SOME DIAMINES USED AS TEMPLATES [J].
MINTOVA, S ;
VALTCHEV, V ;
KANEV, I .
ZEOLITES, 1993, 13 (04) :305-308