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OPTICAL HETERODYNE-DETECTION OF IMPULSIVE STIMULATED RAMAN-SCATTERING IN LIQUIDS

被引：58
作者：
CHANG, YJ
CONG, P
SIMON, JD
机构：
[1] UNIV CALIF SAN DIEGO,DEPT CHEM & BIOCHEM,LA JOLLA,CA 92093
[2] UNIV CALIF SAN DIEGO,INST NONLINEAR SCI,LA JOLLA,CA 92093
来源：
JOURNAL OF PHYSICAL CHEMISTRY | 1995年 / 99卷 / 20期
关键词：
D O I：
10.1021/j100020a004
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Optical heterodyne detection is implemented in an impulsive stimulated Raman scattering (ISRS) experiment by the use of a Mach-Zehnder interferometer. The combination of polarization-selective ISRS and heterodyne detection allows direct measurements of the real and imaginary parts of an arbitrary element of the third-rank material response tenser chi((3)). The heterodyne-detected chi(1111)((3))(t) of CS2 is presented and compared with the homodyne-detected response.
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页码：7857 / 7859
页数：3
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