2-PHOTON ABSORPTION-SPECTROSCOPY OF POLYDIACETYLENE PTS

被引:8
作者
LENG, JM
VARDENY, ZV
HOOPER, BA
STRAUB, KD
MADEY, JMJ
BAKER, GL
机构
[1] DUKE UNIV, FREE ELECTRON LASER LAB, DURHAM, NC 27708 USA
[2] MICHIGAN STATE UNIV, DEPT CHEM, E LANSING, MI 48824 USA
来源
MOLECULAR CRYSTALS AND LIQUID CRYSTALS SCIENCE AND TECHNOLOGY SECTION A-MOLECULAR CRYSTALS AND LIQUID CRYSTALS | 1994年 / 256卷
关键词
D O I
10.1080/10587259408039300
中图分类号
O7 [晶体学];
学科分类号
0702 ; 070205 ; 0703 ; 080501 ;
摘要
We have studied two photon absorption (TPA) of single crystal polydiacetylene-toluene-sulfonate (PTS) using the Mark III Free Electron Laser (FEL) in the spectrum range of 0.95 - 1.5 mu m. We observed two features in the TPA spectrum at two photon energies of 1.85 eV and 2.35 eV, respectively. We discuss the assignment of the two bands in terms of TPA allowed excitons reached by two successive one-photon absorptions.
引用
收藏
页码:617 / 623
页数:7
相关论文
共 14 条
[1]   EXCITONS AND NONLINEAR OPTICAL-SPECTRA IN CONJUGATED POLYMERS [J].
ABE, S ;
SCHREIBER, M ;
SU, WP ;
YU, J .
PHYSICAL REVIEW B, 1992, 45 (16) :9432-9435
[2]  
Etemad S., 1991, SPECTROSCOPY ADV MAT, P87
[3]   ROLE OF THE CONDUCTION-BAND IN ELECTROABSORPTION, 2-PHOTON ABSORPTION, AND 3RD-HARMONIC GENERATION IN POLYDIACETYLENES [J].
GUO, D ;
MAZUMDAR, S ;
DIXIT, SN ;
KAJZAR, F ;
JARKA, F ;
KAWABE, Y ;
PEYGHAMBARIAN, N .
PHYSICAL REVIEW B, 1993, 48 (03) :1433-1459
[4]   LONG-LIFETIME CHARGED PHOTO-EXCITATIONS IN POLYDIACETYLENES - STRONGLY LOCALIZED BIPOLARONS [J].
KIM, YH ;
NOWAK, M ;
SOOS, ZG ;
HEEGER, AJ .
JOURNAL OF PHYSICS C-SOLID STATE PHYSICS, 1988, 21 (15) :L503-L508
[5]  
LENG J, UNPUB
[6]   OPTICAL PROBES OF EXCITED-STATES IN POLY(P-PHENYLENEVINYLENE) [J].
LENG, JM ;
JEGLINSKI, S ;
WEI, X ;
BENNER, RE ;
VARDENY, ZV ;
GUO, F ;
MAZUMDAR, S .
PHYSICAL REVIEW LETTERS, 1994, 72 (01) :156-159
[7]  
NUNZI JM, 1991, NATO ADV SCI I E-APP, V194, P345
[8]   ONE-DIMENSIONAL WIDE ENERGY-BANDS IN A POLYDIACETYLENE REVEALED BY ELECTROREFLECTANCE [J].
SEBASTIAN, L ;
WEISER, G .
PHYSICAL REVIEW LETTERS, 1981, 46 (17) :1156-1159
[9]  
Shen Y.-R., 1984, PRINCIPLES NONLINEAR
[10]  
STEGEMAN G, 1994, MOL CRYST LIQ CRYS A, V256