INELASTIC NEUTRON-SCATTERING MEASUREMENTS OF OPTICAL VIBRATION FREQUENCY-DISTRIBUTIONS IN HYDROGEN-METAL SYSTEMS

被引:69
作者
ROSS, DK
MARTIN, PF
OATES, WA
BAKHSH, RK
机构
[1] Department of Physics, University of Birmingham, Kyushu University
[2] University of Newcastle, New South Wales
来源
ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-WIESBADEN | 1979年 / 114卷
关键词
Density of states; Fluorite structures; Hydrogen metal systems; Neutron energy loss cross section; PdH[!sub]x[!/sub;
D O I
10.1524/zpch.1979.114.114.221
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Neutron energy loss cross section measurements on hydrogen metal systems are reported. Peaks were observed for a number of samples with fluorite structures where the hydrogens are located on regular tetrahedral sites with a view to examining whether factors other than the M – H distance (R) were important. Only small deviations from a correlation E(R) = A R-2/3 were in fact found. Frequency distributions for PdHx. (x = 0.70, 0.85, and 0.93) were also measured. Although the high frequency shoulder on the peak decreased in intensity, the high concentration curve was still far removed from the density of states curve obtained from Born-Von Karman fits to dispersion curves measured for PdD0.63. © by Akademische Verlagsgesellschaft
引用
收藏
页码:221 / 230
页数:10
相关论文
共 19 条
  • [1] INTERSTITIAL INTERACTIONS IN THE PALLADIUM-HYDROGEN (DEUTERIUM) SYSTEM
    ANDERSON, IS
    CARLILE, CJ
    ROSS, DK
    WILSON, DLT
    [J]. ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-WIESBADEN, 1979, 115 (02): : 165 - 175
  • [2] STRUCTURE IN NEUTRON SCATTERING SPECTRA OF ZIRCONIUM HYDRIDE
    COUCH, JG
    HARLING, OK
    CLUNE, LC
    [J]. PHYSICAL REVIEW B, 1971, 4 (08): : 2675 - &
  • [3] OPTICAL PHONONS IN PDHX AND PDDX BY SUPERCONDUCTING TUNNELING MEASUREMENTS
    DUMOULIN, L
    NEDELLEC, P
    ARZOUMANIAN, C
    BURGER, JP
    [J]. PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 1978, 90 (01): : 207 - 210
  • [4] HIGH-FREQUENCY LOCAL MODES, SUPERCONDUCTIVITY AND ANOMALOUS ISOTOPE-EFFECT IN PDH(D) SYSTEMS
    GANGULY, BN
    [J]. ZEITSCHRIFT FUR PHYSIK, 1973, 265 (05): : 433 - 439
  • [5] COORDINATION OF HYDROGEN IN TRANSITION-METAL HYDRIDES
    HAUCK, J
    SCHENK, HJ
    [J]. JOURNAL OF THE LESS-COMMON METALS, 1977, 51 (02): : 251 - 258
  • [6] OPTICAL VIBRATIONS OF HYDROGEN IN METALS
    HUNT, DG
    ROSS, DK
    [J]. JOURNAL OF THE LESS-COMMON METALS, 1976, 49 (1-2): : 169 - 191
  • [7] HUNT DG, 1971, RARE EARTHS ACTINIDE, V3, P46
  • [8] DIFFUSION OF H2, D2, AND T2 IN SINGLE-CRYSTAL NI AND CU
    KATZ, L
    GUINAN, M
    BORG, RJ
    [J]. PHYSICAL REVIEW B-SOLID STATE, 1971, 4 (02): : 330 - &
  • [9] ELECTRONIC MODEL FOR REVERSE ISOTOPE-EFFECT IN SUPERCONDUCTING PD-H(D)
    MILLER, RJ
    SATTERTHWAITE, CB
    [J]. PHYSICAL REVIEW LETTERS, 1975, 34 (03) : 144 - 148
  • [10] PHONON SPECTRA OF NONSTOICHIOMETRIC PALLADIUM HYDRIDES
    RAHMAN, A
    SKOLD, K
    PELIZZARI, C
    SINHA, SK
    FLOTOW, H
    [J]. PHYSICAL REVIEW B, 1976, 14 (08): : 3630 - 3634