ARE THERE REALLY 4 MANGANESE IONS PER CENTER OF PHOTOSYNTHETIC WATER OXIDATION

被引:12
作者
PAULY, S [1 ]
WITT, HT [1 ]
机构
[1] TECH UNIV BERLIN,MAX VOLMER INST BIOPHYS & PHYS CHEM,STR DES 17 JUNI 135,W-1000 BERLIN 12,GERMANY
关键词
PHOTOSYNTHESIS; OXYGEN EVOLUTION; MANGANESE; (SYNECHOCOCCUS);
D O I
10.1016/0005-2728(92)90029-2
中图分类号
Q5 [生物化学]; Q7 [分子生物学];
学科分类号
071010 ; 081704 ;
摘要
Manganese content and the amount of oxygen-evolving centres have determined for purified PS II complexes from the cyanobacterium Synechococcus sp. by atomic absorption and measurements of flash-induced oxygen yields, respectively. A stoichiometry of six manganese per oxygen-evolving centre was observed. This was found not only for PS II preparations with different activities of oxygen evolution, but also when deactivating treatments by low-salt or NH2OH incubation were carried out. Our results call into question the current thinking that four Mn ions are located in the water-oxidizing complex. A hexanuclear manganese model is discussed, instead.
引用
收藏
页码:211 / 218
页数:8
相关论文
共 63 条
[1]   A COMPARISON BETWEEN THE MULTILINE ELECTRON-PARAMAGNETIC-RES SIGNALS OF SPINACH AND ANACYSTIS-NIDULANS AND THEIR TEMPERATURE-DEPENDENCE [J].
AASA, R ;
ANDREASSON, LE ;
LAGENFELT, G ;
VANNGARD, T .
FEBS LETTERS, 1987, 221 (02) :245-248
[3]  
ABRAMOWICZ DA, 1984, ADV PHOTOSYNTHESIS R, V1, P349
[4]   THE ROLE OF MANGANESE IN PHOTOSYNTHETIC OXYGEN EVOLUTION [J].
AMESZ, J .
BIOCHIMICA ET BIOPHYSICA ACTA, 1983, 726 (01) :1-12
[5]   PREPARATION, CRYSTAL-STRUCTURE, MAGNETIC-PROPERTIES, AND CHEMICAL-REACTIONS OF A HEXANUCLEAR MIXED-VALENCE MANGANESE CARBOXYLATE [J].
BAIKIE, ARE ;
HOWES, AJ ;
HURSTHOUSE, MB ;
QUICK, AB ;
THORNTON, P .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1986, (21) :1587-1587
[6]   MANGANESE IN PHOTOSYNTHETIC OXYGEN EVOLUTION .1. ELECTRON-PARAMAGNETIC RESONANCE STUDY OF ENVIRONMENT OF MANGANESE IN TRIS-WASHED CHLOROPLASTS [J].
BLANKENSHIP, RE ;
SAUER, K .
BIOCHIMICA ET BIOPHYSICA ACTA, 1974, 357 (02) :252-266
[7]   THE TETRANUCLEAR MANGANESE COMPLEX OF PHOTOSYSTEM-II [J].
BRUDVIG, GW .
JOURNAL OF BIOENERGETICS AND BIOMEMBRANES, 1987, 19 (02) :91-104
[8]  
CHENIAE G, 1980, METHOD ENZYMOL, V69, P349
[9]   SITES OF FUNCTION OF MANGANESE WITHIN PHOTOSYSTEM-II - ROLES IN O2 EVOLUTION AND SYSTEM-II [J].
CHENIAE, GM ;
MARTIN, IF .
BIOCHIMICA ET BIOPHYSICA ACTA, 1970, 197 (02) :219-&
[10]   EFFECTS OF HYDROXYLAMINE ON PHOTOSYSTEM-II .1. FACTORS AFFECTING DECAY OF O2 EVOLUTION [J].
CHENIAE, GM ;
MARTIN, IF .
PLANT PHYSIOLOGY, 1971, 47 (04) :568-&