ANOMALOUS DIFFUSION IN ELONGATED MICELLES AND ITS LEVY FLIGHT INTERPRETATION

被引:76
作者
BOUCHAUD, JP
OTT, A
LANGEVIN, D
URBACH, W
机构
[1] UNIV PARIS 06, PHYS STAT LAB, F-75231 PARIS 5, FRANCE
[2] UNIV PARIS 07, PHYS STAT LAB, F-75231 PARIS 5, FRANCE
来源
JOURNAL DE PHYSIQUE II | 1991年 / 1卷 / 12期
关键词
D O I
10.1051/jp2:1991163
中图分类号
O3 [力学];
学科分类号
08 ; 0801 ;
摘要
We have observed anomalously enhanced self (tracer) diffusion in systems of polymer-like, breakable micelles. We argue that it provides the first experimental realization of a random walk for which the second moment of the jump size distribution fails to exist (<< Levy-flight >>). The basic mechanism is the following: due to reptation, short micelles diffuse much more rapidly than long ones. As time goes on, shorter and shorter micelles are encountered by the tracer, and hence the effective diffusion constant increases with time. We discuss in detail the fact that this anomalous regime only exists in a certain range of concentration and temperature. The theoretical dependence of the asymptotic diffusion constant on concentration is in quite good agreement with the experiment.
引用
收藏
页码:1465 / 1482
页数:18
相关论文
共 43 条
[1]   RENORMALIZATION-GROUP APPROACH TO NONCOHERENT RADIATIVE-TRANSFER [J].
BELL, TL ;
FRISCH, U ;
FRISCH, H .
PHYSICAL REVIEW A, 1978, 17 (03) :1049-1057
[2]  
BERNASCONI J, 1979, PHYS REV LETT, V41, P185
[3]   SUPERDIFFUSION IN RANDOM VELOCITY-FIELDS [J].
BOUCHAUD, JP ;
GEORGES, A ;
KOPLIK, J ;
PROVATA, A ;
REDNER, S .
PHYSICAL REVIEW LETTERS, 1990, 64 (21) :2503-2506
[4]   ANOMALOUS DIFFUSION IN DISORDERED MEDIA - TRAPPING, CORRELATIONS AND THE CENTRAL-LIMIT-THEOREM [J].
BOUCHAUD, JP ;
GEORGES, A ;
LEDOUSSAL, P .
JOURNAL DE PHYSIQUE, 1987, 48 (11) :1855-1860
[5]   ANOMALOUS DIFFUSION IN DISORDERED MEDIA - STATISTICAL MECHANISMS, MODELS AND PHYSICAL APPLICATIONS [J].
BOUCHAUD, JP ;
GEORGES, A .
PHYSICS REPORTS-REVIEW SECTION OF PHYSICS LETTERS, 1990, 195 (4-5) :127-293
[6]  
BOUCHAUD JP, UNPUB
[7]  
CANDAU J, 1988, J COLLOID INTERF SCI, V122, P430
[8]   NEW ASPECTS OF THE BEHAVIOR OF ALKYLTRIMETHYLAMMONIUM BROMIDE MICELLES - LIGHT-SCATTERING AND VISCOSIMETRIC STUDIES [J].
CANDAU, SJ ;
HIRSCH, E ;
ZANA, R .
JOURNAL DE PHYSIQUE, 1984, 45 (07) :1263-1270
[9]   TEMPERATURE-JUMP STUDY OF ELONGATED MICELLES OF CETYLTRIMETHYLAMMONIUM BROMIDE [J].
CANDAU, SJ ;
MERIKHI, F ;
WATON, G ;
LEMARECHAL, P .
JOURNAL DE PHYSIQUE, 1990, 51 (10) :977-989
[10]   LIGHT-SCATTERING INVESTIGATIONS OF THE BEHAVIOR OF SEMIDILUTE AQUEOUS MICELLAR SOLUTIONS OF CETYLTRIMETHYLAMMONIUM BROMIDE - ANALOGY WITH SEMIDILUTE POLYMER-SOLUTIONS [J].
CANDAU, SJ ;
HIRSCH, E ;
ZANA, R .
JOURNAL OF COLLOID AND INTERFACE SCIENCE, 1985, 105 (02) :521-528