EXCITONIC INTERACTIONS IN THE LIGHT-HARVESTING ANTENNA OF PHOTOSYNTHETIC PURPLE BACTERIA AND THEIR INFLUENCE ON PICOSECOND ABSORBENCY DIFFERENCE SPECTRA

被引:65
作者
NOVODEREZHKIN, VI
RAZJIVIN, AP
机构
[1] AN BELOZERSKY PHYS CHEM BIOL INST,DEPT PHOTOSYNTHESIS,BLDG A,MOSCOW 119899,RUSSIA
[2] MOSCOW MV LOMONOSOV STATE UNIV,CTR INT LASER,MOSCOW 119899,RUSSIA
[3] RUSSIAN ACAD SCI,TECHNOL LASERS RES CTR,MOSCOW 142092,RUSSIA
关键词
EXCITONIC INTERACTION; PICOSECOND ABSORBENCY DIFFERENCE SPECTRUM; BACTERIAL PHOTOSYNTHESIS; LIGHT-HARVESTING ANTENNA;
D O I
10.1016/0014-5793(93)80907-C
中图分类号
Q5 [生物化学]; Q7 [分子生物学];
学科分类号
071010 ; 081704 ;
摘要
A new model of the light-harvesting antenna (core complex) of purple photosynthetic bacteria is proposed based on excitonic interactions in circular aggregates of bacteriochlorophyll molecules. The calculated absorbance difference spectra of circular aggregates demonstrate all special features observed in the experimental spectra of purple bacteria. In particular, the absorption changes with high amplitude of bleaching at the long-wavelength side of the absorption band at different excitation energy are predicted.
引用
收藏
页码:5 / 7
页数:3
相关论文
共 16 条
[1]  
ABDOURAKHMANOV IA, 1986, 7TH INT C PHOT, P303
[2]   ENERGY-TRANSFER WITHIN THE ISOLATED B875 LIGHT-HARVESTING PIGMENT-PROTEIN COMPLEX OF RHODOBACTER-SPHAEROIDES AT 77-K STUDIED BY PICOSECOND ABSORPTION-SPECTROSCOPY [J].
BERGSTROM, H ;
WESTERHUIS, WHJ ;
SUNDSTROM, V ;
VANGRONDELLE, R ;
NIEDERMAN, RA ;
GILLBRO, T .
FEBS LETTERS, 1988, 233 (01) :12-16
[3]   MINOR COMPONENT B-905 OF LIGHT-HARVESTING ANTENNA IN RHODOSPIRILLUM-RUBRUM CHROMATOPHORES AND THE MECHANISM OF SINGLET-SINGLET ANNIHILATION AS STUDIED BY DIFFERENCE SELECTIVE PICOSECOND SPECTROSCOPY [J].
BORISOV, AY ;
GADONAS, RA ;
DANIELIUS, RV ;
PISKARSKAS, AS ;
RAZJIVIN, AP .
FEBS LETTERS, 1982, 138 (01) :25-28
[4]   FERMION BEHAVIOR OF 1-DIMENSIONAL EXCITONS [J].
CHESNUT, DB ;
SUNA, A .
JOURNAL OF CHEMICAL PHYSICS, 1963, 39 (01) :146-&
[5]   THE COOPERATIVITY PHENOMENA IN A PIGMENT-PROTEIN COMPLEX OF LIGHT-HARVESTING ANTENNA REVEALED BY PICOSECOND ABSORBANCE DIFFERENCE SPECTROSCOPY [J].
DANIELIUS, RV ;
MINEYEV, AP ;
RAZJIVIN, AP .
FEBS LETTERS, 1989, 250 (02) :183-186
[6]   ENERGY-TRANSFER DYNAMICS IN 3 LIGHT-HARVESTING MUTANTS OF RHODOBACTER-SPHAEROIDES - A PICOSECOND SPECTROSCOPY STUDY [J].
HUNTER, CN ;
BERGSTROM, H ;
VANGRONDELLE, R ;
SUNDSTROM, V .
BIOCHEMISTRY, 1990, 29 (13) :3203-3207
[7]  
NOVODEREZHKIN VI, 1993, IN PRESS 4TH P INT C
[8]  
NOVODEREZHKIN VI, 1992, 4TH INT C LAS APPL L, P175
[9]   SINGLET AND TRIPLET EXCITED CAROTENOID AND ANTENNA BACTERIOCHLOROPHYLL OF THE PHOTOSYNTHETIC PURPLE BACTERIUM RHODOSPIRILLUM-RUBRUM AS STUDIED BY PICOSECOND ABSORBANCE DIFFERENCE SPECTROSCOPY [J].
NUIJS, AM ;
VANGRONDELLE, R ;
JOPPE, HLP ;
VANBOCHOVE, AC ;
DUYSENS, LNM .
BIOCHIMICA ET BIOPHYSICA ACTA, 1985, 810 (01) :94-105
[10]   PICOSECOND FLUORESCENCE OF SIMPLE PHOTOSYNTHETIC MEMBRANES - EVIDENCE OF SPECTRAL INHOMOGENEITY AND DIRECTED ENERGY-TRANSFER [J].
PULLERITS, T ;
FREIBERG, A .
CHEMICAL PHYSICS, 1991, 149 (03) :409-418