THE REACTION OF CO2 WITH CH4 TO SYNTHESIZE H-2 AND CO OVER NICKEL-LOADED Y-ZEOLITES

被引:86
作者
KIM, GJ
CHO, DS
KIM, KH
KIM, JH
机构
[1] INHA JR TECH COLL,DEPT IND CHEM,INCHON 402751,SOUTH KOREA
[2] TOKYO INST TECHNOL,DEPT CHEM,MEGURO KU,TOKYO 152,JAPAN
关键词
NICKEL; Y-ZEOLITE; ION EXCHANGE; HYDROGENATION OF CARBON DIOXIDE; METHANE; HYDROGEN; CARBON MONOXIDE; ACID STRENGTH; ELECTROSTATIC FIELD;
D O I
10.1007/BF00812468
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Nickel metal introduced into Y-zeolite exhibited a high catalytic activity in the dehydrogenation of methane and in the hydrogenation of carbon dioxide with methane to obtain hydrogen and CO at about 850 K. The activity strongly depended on the nickel amount in NaY, and the catalytic properties were influenced by the kind of cations in the Y-zeolite. The higher CO2 conversion was obtained over Ni supported on non-acidic zeolites.
引用
收藏
页码:41 / 52
页数:12
相关论文
共 24 条
[11]  
KIM GJ, 1987, J KOREAN I CHEM ENG, V25, P477
[12]  
KNEALE B, 1983, FARADAY T 1, V79, P157
[13]   REACTIONS OF CO AND CO2 ON NI-SIO2 ABOVE 373-K AS STUDIED BY INFRARED SPECTROSCOPIC AND MAGNETIC METHODS [J].
MARTIN, GA ;
PRIMET, M ;
DALMON, JA .
JOURNAL OF CATALYSIS, 1978, 53 (03) :321-330
[14]   HYDROGENATION OF SURFACE CARBON ON ALUMINA-SUPPORTED NICKEL [J].
MCCARTY, JG ;
WISE, H .
JOURNAL OF CATALYSIS, 1979, 57 (03) :406-416
[15]  
NAKAMURA J, 1991, SHOKUBAI, V33, P99
[16]  
PARK DS, 1989, J KOREAN I CHEM ENG, V27, P723
[17]  
Rostrup-Nielsen J. R., 1984, CATALYSIS SCI TECHNO, V5, DOI DOI 10.1007/978-3-642-93247-2_
[18]  
ROSTRUPNIELSEN J, 1988, METHANE CONVERSION, P73
[19]  
SATTERFIELD CN, 1980, HETEROGENEOUS CATALY, P280
[20]  
SAUVION GN, 1982, STUDIES SURFACE SCI, V12, P229