COMPLEX-SCALING FOURIER-GRID HAMILTONIAN METHOD .3. OSCILLATORY BEHAVIOR OF COMPLEX QUASI-ENERGIES AND THE STABILITY OF NEGATIVE-IONS IN VERY INTENSE LASER FIELDS

被引:59
作者
YAO, GH
CHU, SI
机构
[1] Department of Chemistry, University of Kansas, Lawrence
来源
PHYSICAL REVIEW A | 1992年 / 45卷 / 09期
关键词
D O I
10.1103/PhysRevA.45.6735
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
A complex-scaling Fourier-grid Hamiltonian (CSFGH) method in momentum representation along with Floquet formalism is presented and applied to the nonperturbative treatment of the complex quasienergies of a one-dimensional-model negative chlorine ion in an ArF excimer-laser field. The CSFGH method leads to a simple and highly efficient variational procedure for accurate determination of resonance states, without the need of using an L2-basis-function expansion. A variety of laser intensities are considered covering those from perturbative to very intense laser fields, and the stability of the ion is investigated under realistic experimental conditions. Oscillatory structures of the photodetachment rate as a function of field strength are found in our study, revealing that the decreasing of the detachment rate (or the so-called "stabilization" or "suppression-of-ionization" phenomenon) may not necessarily be a monotonic behavior. Physical insight into this interesting feature is explored in the Kramers-Henneberger frame, and the feasibility for the experimental observation of the oscillatory behavior of the negative ions is also discussed.
引用
收藏
页码:6735 / 6743
页数:9
相关论文
共 26 条
[1]   MULTIPHOTON IONIZATION FROM A SHORT-RANGE POTENTIAL BY SHORT-PULSE LASERS [J].
BARDSLEY, JN ;
SZOKE, A ;
COMELLA, MJ .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1988, 21 (23) :3899-3916
[2]   AC STARK-EFFECT FOR SHORT-RANGE POTENTIALS WITH INTENSE ELECTROMAGNETIC-FIELDS [J].
BARDSLEY, JN ;
COMELLA, MJ .
PHYSICAL REVIEW A, 1989, 39 (04) :2252-2255
[3]   SUPPRESSION OF IONIZATION IN STRONG LASER FIELDS [J].
BURNETT, K ;
KNIGHT, PL ;
PIRAUX, BRM ;
REED, VC .
PHYSICAL REVIEW LETTERS, 1991, 66 (03) :301-304
[4]  
Chu S, 1989, ADV CHEM PHYS, V73, P739
[5]   THE COMPLEX-SCALING FOURIER-GRID HAMILTONIAN METHOD FOR RESONANCE STATE PROBLEMS [J].
CHU, SI .
CHEMICAL PHYSICS LETTERS, 1990, 167 (1-2) :155-157
[6]   RECENT DEVELOPMENTS IN SEMICLASSICAL FLOQUET THEORIES FOR INTENSE-FIELD MULTIPHOTON PROCESSES [J].
CHU, SI .
ADVANCES IN ATOMIC AND MOLECULAR PHYSICS, 1985, 21 :197-253
[7]   COMPLEX QUASIVIBRATIONAL ENERGY FORMALISM FOR INTENSE-FIELD MULTIPHOTON AND ABOVE-THRESHOLD DISSOCIATION - COMPLEX-SCALING FOURIER-GRID HAMILTONIAN METHOD [J].
CHU, SI .
JOURNAL OF CHEMICAL PHYSICS, 1991, 94 (12) :7901-7909
[8]   MULTIPHOTON PROCESSES IN AN INTENSE LASER FIELD .5. THE HIGH-FREQUENCY REGIME [J].
DORR, M ;
POTVLIEGE, RM ;
PROULX, D ;
SHAKESHAFT, R .
PHYSICAL REVIEW A, 1991, 43 (07) :3729-3740
[9]   FREE-FREE TRANSITIONS IN INTENSE HIGH-FREQUENCY LASER FIELDS [J].
GAVRILA, M ;
KAMINSKI, JZ .
PHYSICAL REVIEW LETTERS, 1984, 52 (08) :613-616
[10]   PERTURBATION METHOD FOR ATOMS IN INTENSE LIGHT BEAMS [J].
HENNEBERGER, WC .
PHYSICAL REVIEW LETTERS, 1968, 21 (12) :838-+