OPTICAL NONLINEARITIES IN SUBSTITUTED SYMMETRIC CYANINE DYES

被引:23
作者
MEHENDALE, SC
RUSTAGI, KC
机构
[1] Laser Section, Bhabha Atomic Research Centre, Bombay, 85, Trombay
关键词
D O I
10.1016/0030-4018(79)90339-0
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Linear and third order polarizabilities for aza-derivatives of symmetric cyanine dyes are calculated in a free-electron like model. The nonlinearity in these molecules is larger compared to the corresponding cyanines and polyenes. This is attributed to the N-atom substitution causing an increased anharmonicity without significantly reducing the delocalization. © 1979.
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页码:359 / 362
页数:4
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