SIGN OF CHI(3) IN POLYSILANE POLYMERS

被引:25
作者
YANG, L
DORSINVILLE, R
ALFANO, RR
ZOU, WK
YANG, NL
机构
[1] CUNY CITY COLL,DEPT PHYS,NEW YORK,NY 10031
[2] CUNY COLL STATEN ISL,DEPT CHEM,STATEN ISL,NY 10301
关键词
D O I
10.1364/OL.16.000758
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The signs of the third-order optical nonlinear susceptibility chi(3) of polysilane have been determined to be negative at 532 nm and positive at 1064 nm from single-beam Z-scan measurements. The small and positive chi(3) at 1064 nm arises from the bound-electronic process. The negative chi(3) at 532 nm is attributed to two-photon absorption resonance transition.
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收藏
页码:758 / 760
页数:3
相关论文
共 17 条
[1]   TEMPERATURE-DEPENDENCE OF THE 3RD-ORDER NONLINEAR OPTICAL SUSCEPTIBILITIES IN POLYSILANES AND POLYGERMANES [J].
BAUMERT, JC ;
BJORKLUND, GC ;
JUNDT, DH ;
JURICH, MC ;
LOOSER, JH ;
MILLER, RD ;
RABOLT, J ;
SOORIYAKUMARAN, R ;
SWALEN, JD ;
TWIEG, RJ .
APPLIED PHYSICS LETTERS, 1988, 53 (13) :1147-1149
[2]  
Bloembergen N., 1965, NONLINEAR OPTICS
[3]  
FLYTZANIS C, 1975, QUANTUM ELECTRON, V1, P9
[4]  
KAZJAR F, 1986, J APPL PHYS, V60, P3040
[5]  
KEPLER RG, 1990, MATER RES SOC SYMP P, V173, P453
[6]  
KEPLER RG, 1990, ADV CHEM SERIES, V224
[7]  
Mahr H., 1975, QUANTUM ELECTRON, P285
[8]   RESOLUTION OF THE NUCLEAR AND ELECTRONIC CONTRIBUTIONS TO THE OPTICAL NONLINEARITY IN POLYSILANES [J].
MCGRAW, DJ ;
SIEGMAN, AE ;
WALLRAFF, GM ;
MILLER, RD .
APPLIED PHYSICS LETTERS, 1989, 54 (18) :1713-1715
[9]   2-PHOTON-INDUCED BIREFRINGENCE IN POLYSILANES [J].
SCHELLENBERG, FM ;
BYER, RL ;
MILLER, RD .
CHEMICAL PHYSICS LETTERS, 1990, 166 (04) :331-339
[10]   FABRICATION OF BIREFRINGENT GRATINGS USING NONLINEAR POLYSILANE THIN-FILMS [J].
SCHELLENBERG, FM ;
BYER, RL ;
MILLER, RD .
OPTICS LETTERS, 1990, 15 (04) :242-244