A COMPARISON OF THE PREDICTIONS OF AN EULERIAN ATMOSPHERIC TRANSPORT - CHEMISTRY MODEL WITH EXPERIMENTAL MEASUREMENTS OVER THE NORTH-SEA

被引:34
作者
HARRISON, RM
ZLATV, Z
OTTLEY, CJ
机构
[1] MINIST ENVIRONM,NATL ENVIRONM RES INST,DK-4000 ROSKILDE,DENMARK
[2] UNIV LANCASTER,DEPT ENVIRONM SCI,LANCASTER LA1 4YQ,ENGLAND
关键词
MEASUREMENTS; ATMOSPHERIC MODELS; CONCENTRATIONS OF AIR POLLUTANTS; ATMOSPHERIC TRANSPORT; CHEMICAL REACTIONS; DIFFUSION; DEPOSITION; EMISSIONS;
D O I
10.1016/1352-2310(94)90127-9
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
A very comprehensive set of airborne concentration measurements for gaseous HNO3 and NH3 and particulate NH4+, SO4(2-) and NO3- collected abroad R.R.S. Challenger over the Southern Bight of the North Sea has been compared with the predictions of an Eulerian atmospheric transport-chemistry model. Comparison of time-averaged concentrations and temporal variations shows generally excellent agreement between measurements and model predictions. It is concluded that, given the difficulties of making airborne concentration measurements over the Sea, the model provides a reliable and cost-effective means of estimating pollutant concentrations.
引用
收藏
页码:497 / 516
页数:20
相关论文
共 62 条
[11]  
DEDEURWAERDER HL, 1983, PRECIPITATION SCAVEN, V2, P1219
[12]  
EBEL A, 1991, P EMEP WORKSHOP PHOT, P142
[13]  
ELIASSEN A, 1982, J APPL METEOROL, V21, P1645, DOI 10.1175/1520-0450(1982)021<1645:ALLRTM>2.0.CO
[14]  
2
[15]  
Gear CW., 1971, NUMERICAL INITIAL VA
[16]   A PHOTOCHEMICAL KINETICS MECHANISM FOR URBAN AND REGIONAL SCALE COMPUTER MODELING [J].
GERY, MW ;
WHITTEN, GZ ;
KILLUS, JP ;
DODGE, MC .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1989, 94 (D10) :12925-12956
[17]   HORIZONTAL DIFFUSION IN THE ATMOSPHERE - A LAGRANGIAN-DYNAMICAL THEORY [J].
GIFFORD, FA .
ATMOSPHERIC ENVIRONMENT, 1982, 16 (03) :505-512
[18]  
GRENNFELT P, 1986, NORDISK MINISTERRAD, V18
[19]  
HANNA SR, 1985, AIR POLLUTION MODELL, V5, P441
[20]   ESTIMATION OF THE RATE-CONSTANT FOR THE REACTION OF ACID SULFATE AEROSOL WITH NH3 GAS FROM ATMOSPHERIC MEASUREMENTS [J].
HARRISON, RM ;
KITTO, AMN .
JOURNAL OF ATMOSPHERIC CHEMISTRY, 1992, 15 (02) :133-143