C-13 NMR-STUDY OF LAYERED ORGANIC SUPERCONDUCTORS BASED ON BEDT-TTF MOLECULES

被引:175
作者
KAWAMOTO, A [1 ]
MIYAGAWA, K [1 ]
NAKAZAWA, Y [1 ]
KANODA, K [1 ]
机构
[1] INST MOLEC SCI,OKAZAKI,AICHI 444,JAPAN
关键词
D O I
10.1103/PhysRevLett.74.3455
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The normal state of the layered organic superconductors κ-(BEDT-TTF)2X (X=Cu(NCS)2 and Cu[N(CN)2]Br) has been studied by 13C NMR for the first time. The nuclear spin-lattice relaxation rate, T1-1, is greatly enhanced over the value expected from the Korringa relation and shows an anomalous peak around 50 K for both compounds. This is the first experimental evidence of strong antiferromagnetic spin fluctuations in these materials. The depression of the spin fluctuations observed below 50 K coincides with an appearance of Fermi liquid behavior in the charge transport. © 1995 The American Physical Society.
引用
收藏
页码:3455 / 3458
页数:4
相关论文
共 19 条
  • [1] MAGNETOTRANSPORT STUDIES OF THE ORGANIC SUPERCONDUCTOR KAPPA-(BEDT-TTF)2CU(NCS)2 UNDER PRESSURE - THE RELATIONSHIP BETWEEN CARRIER EFFECTIVE-MASS AND CRITICAL-TEMPERATURE
    CAULFIELD, J
    LUBCZYNSKI, W
    PRATT, FL
    SINGLETON, J
    KO, DYK
    HAYES, W
    KURMOO, M
    DAY, P
    [J]. JOURNAL OF PHYSICS-CONDENSED MATTER, 1994, 6 (15) : 2911 - 2924
  • [2] EVIDENCE FOR THE ROLE OF FLUXOIDS IN ENHANCING NMR SPIN-LATTICE RELAXATION AND IMPLICATIONS FOR INTRINSIC PINNING OF THE FLUX LATTICE IN ORGANIC SUPERCONDUCTORS
    DESOTO, SM
    SLICHTER, CP
    WANG, HH
    GEISER, U
    WILLIAMS, JM
    [J]. PHYSICAL REVIEW LETTERS, 1993, 70 (19) : 2956 - 2959
  • [3] NMR-STUDY OF AN ORGANIC SUPERCONDUCTOR, KAPPA-(BEDT-TTF)2CU[N(CN)2]BR
    KANODA, K
    SAKAO, K
    TAKAHASHI, T
    KOMATSU, T
    SAITO, G
    [J]. PHYSICA C, 1991, 185 : 2667 - 2668
  • [4] A NEW AMBIENT-PRESSURE ORGANIC SUPERCONDUCTOR, KAPPA-(ET)2CU[N(CN)2]BR, WITH THE HIGHEST TRANSITION-TEMPERATURE YET OBSERVED (INDUCTIVE ONSET TC = 11.6 K, RESISTIVE ONSET = 12.5 K)
    KINI, AM
    GEISER, U
    WANG, HH
    CARLSON, KD
    WILLIAMS, JM
    KWOK, WK
    VANDERVOORT, KG
    THOMPSON, JE
    STUPKA, DL
    JUNG, D
    WHANGBO, MH
    [J]. INORGANIC CHEMISTRY, 1990, 29 (14) : 2555 - 2557
  • [5] LARSEN J, 1989, SYNTHESIS-STUTTGART, P134
  • [6] CRYSTAL AND ELECTRONIC-STRUCTURES OF (BEDT-TTF)2(KHG(SCN)4), (BEDT-TTF)2(NH4HG(SCN)4)
    MORI, H
    TANAKA, S
    OSHIMA, M
    SAITO, G
    MORI, T
    MARUYAMA, Y
    INOKUCHI, H
    [J]. BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 1990, 63 (08) : 2183 - 2190
  • [7] TEMPERATURE-DEPENDENCE OF HALL-EFFECT IN KAPPA-(BEDT-TTF)2CU(NCS)2
    MURATA, K
    ISHIBASHI, M
    HONDA, Y
    FORTUNE, NA
    TOKUMOTO, M
    KINOSHITA, N
    ANZAI, H
    [J]. SOLID STATE COMMUNICATIONS, 1990, 76 (03) : 377 - 381
  • [8] SUPERCONDUCTIVITY OF BEDT-TTF SALTS .1. EFFECT, OF PRESSURE AND ALLOYING AND .2. SHUBNIKOV DEHAAS EFFECT
    MURATA, K
    TOKUMOTO, M
    ANZAI, H
    HONDA, Y
    KINOSHITA, N
    ISHIGURO, T
    TOYOTA, N
    SASAKI, T
    MUTO, Y
    [J]. SYNTHETIC METALS, 1988, 27 (1-2) : A263 - A270
  • [9] SYSTEMATIC INVESTIGATION OF ELECTRONIC-STRUCTURE IN BEDT-TTF BASED ORGANIC SUPERCONDUCTORS WITH T(C) ABOVE 10-K - KAPPA-(BEDT-TTF)2X (X=CU(NCS)2, CU[N(CN)2]BR, AND CU(CN)[N(CN)2])
    NAKAMURA, T
    NOBUTOKI, T
    MIYAMOTO, M
    TSUBOKURA, Y
    TSUCHIYA, R
    TAKAHASHI, T
    KANODA, K
    SAITO, G
    [J]. JOURNAL OF SUPERCONDUCTIVITY, 1994, 7 (03): : 671 - 674
  • [10] PRESSURE-TEMPERATURE PHASE-DIAGRAM, INVERSE ISOTOPE EFFECT, AND SUPERCONDUCTIVITY IN EXCESS OF 13-K IN KAPPA-(BEDT-TTF)2CU[N(CN)2]CL, WHERE BEDT-TTF IS BIS(ETHYLENEDITHIO)TETRATHIAFULVALENE
    SCHIRBER, JE
    OVERMYER, DL
    CARLSON, KD
    WILLIAMS, JM
    KINI, AM
    WANG, HH
    CHARLIER, HA
    LOVE, BJ
    WATKINS, DM
    YACONI, GA
    [J]. PHYSICAL REVIEW B, 1991, 44 (09): : 4666 - 4666