POLYCYCLIC AROMATIC-HYDROCARBONS AND MERCURY IN SEDIMENTS FROM 2 ISOLATED LAKES IN CENTRAL AND NORTHERN CANADA

被引:20
作者
LOCKHART, WL [1 ]
WILKINSON, P [1 ]
BILLECK, BN [1 ]
BRUNSKILL, GJ [1 ]
HUNT, RV [1 ]
WAGEMANN, R [1 ]
机构
[1] AUSTRALIAN INST MARINE SCI,TOWNSVILLE,QLD 4810,AUSTRALIA
关键词
SEDIMENT; POLYCYCLIC AROMATIC HYDROCARBONS; MERCURY; CULTURAL ENRICHMENT;
D O I
10.2166/wst.1993.0602
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Sediment cores were taken from two isolated Canadian lakes, a southern lake in the boreal forest region of northwestern Ontario and a northern one in the tundra on the west coast of Hudson Bay for the purpose of comparing current and historical loading of several contaminants. are no sources of anthropogenic contaminants within either basin, yet both lakes showed in polycyclic aromatic hydrocarbon and mercury in more recent sediments as compared with older, deeper sediments. We have interpreted these as indications of increased loadings as a result of atmospheric fallout. When compared on the basis of the sum of sixteen PAHs, both lakes showed peak inputs in the middle years of this century, followed by mom recent declines; although current values still exceed those from deep slices. With respect to mercury, the concentrations found in the southern lake were somewhat higher than those in the northern lake, and loadings were clearly greater in the south. Both lakes showed enrichment of mercury in top layers of the cores relative to bottom layers, and this enrichment was proportionately greater in the north. Both mercury profiles showed a slow mte of increase for a long period before 1850, suggesting influences from areas industrialized before North America. The northern showed increases in PAH loadings prior to 1850, but the southern lake did not.
引用
收藏
页码:43 / 52
页数:10
相关论文
共 24 条
[1]  
BOEHM PD, 1983, CAN J FISH AQUAT SCI, V40, P262
[2]   HIGH-LEVELS OF PCBS IN BREAST-MILK OF INUIT WOMEN FROM ARCTIC QUEBEC [J].
DEWAILLY, E ;
NANTEL, A ;
WEBER, JP ;
MEYER, F .
BULLETIN OF ENVIRONMENTAL CONTAMINATION AND TOXICOLOGY, 1989, 43 (05) :641-646
[3]  
FISK JF, 1986, SPECTRA, V10, P22
[4]   DETERMINATION OF LOW LEVELS OF POLONIUM-210 IN ENVIRONMENTAL MATERIALS [J].
FLYNN, WW .
ANALYTICA CHIMICA ACTA, 1968, 43 (02) :221-&
[5]   DETERMINATION OF POLYCYCLIC AROMATIC-HYDROCARBONS IN ENVIRONMENT BY GLASS CAPILLARY GAS-CHROMATOGRAPHY [J].
GIGER, W ;
SCHAFFNER, C .
ANALYTICAL CHEMISTRY, 1978, 50 (02) :243-249
[6]   FLUXES OF POLYCYCLIC AROMATIC-HYDROCARBONS TO MARINE AND LACUSTRINE SEDIMENTS IN THE NORTHEASTERN UNITED-STATES [J].
GSCHWEND, PM ;
HITES, RA .
GEOCHIMICA ET COSMOCHIMICA ACTA, 1981, 45 (12) :2359-2367
[7]   DETERMINATION OF MERCURY IN FISH [J].
HENDZEL, MR ;
JAMIESON, DM .
ANALYTICAL CHEMISTRY, 1976, 48 (06) :926-928
[8]   CHRONOLOGY AND SOURCES OF ANTHROPOGENIC TRACE-METALS IN SEDIMENTS FROM SMALL, SHALLOW ARCTIC LAKES [J].
HERMANSON, MH .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1991, 25 (12) :2059-2064
[9]  
HERMANSON MH, 1994, WAT SCI TECH, V28
[10]  
Johansson K., 1985, VERH INT VER THEOR A, V22, P2359