THE BOSON PEAK IN GLASS FORMERS OF INCREASING FRAGILITY

被引:85
作者
HASSAN, AK [1 ]
BORJESSON, L [1 ]
TORELL, LM [1 ]
机构
[1] CHALMERS UNIV TECHNOL,DEPT PHYS,S-41296 GOTHENBURG,SWEDEN
关键词
D O I
10.1016/0022-3093(94)90427-8
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The 'universal' low frequency vibrational behaviour of glasses has been investigated for systems of increased fragility. A dynamical correlation length, l(c), was determined from the position of the boson peak in low frequency Raman spectra. It is found that the value of l(c) correlates with the fragility, hence with the relaxation dynamics which characterise the system in the liquid-glass transition range. Results for oxide, ionic and molecular glasses show that l(c) decreases as the fragility of the system increases.
引用
收藏
页码:154 / 160
页数:7
相关论文
共 45 条
[11]   STRUCTURAL RELAXATION IN VITREOUS SILICA [J].
BUCHENAU, U ;
ZHOU, HM ;
NUCKER, N ;
GILROY, KS ;
PHILLIPS, WA .
PHYSICAL REVIEW LETTERS, 1988, 60 (13) :1318-1321
[12]  
BUCHENAU U, 1989, DYNAMICS DISORDERED
[13]   SHORT-RANGE ORDER AND GLASS-TRANSITION IN AGI-AG2O-B2O3 VITREOUS ELECTROLYTES [J].
CHIODELLI, G ;
MAGISTRIS, A ;
VILLA, M ;
BJORKSTAM, JL .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 1982, 51 (02) :143-159
[14]   LITHIUM BORATE GLASSES - A QUANTITATIVE STUDY OF STRENGTH AND FRAGILITY [J].
CHRYSSIKOS, GD ;
DUFFY, JA ;
HUTCHINSON, JM ;
INGRAM, MD ;
KAMITSOS, EI ;
PAPPIN, AJ .
JOURNAL OF NON-CRYSTALLINE SOLIDS, 1994, 172 (pt 1) :378-383
[15]   VIBRATIONAL DYNAMICS AND THE STRUCTURE OF GLASSES [J].
DUVAL, E ;
BOUKENTER, A ;
ACHIBAT, T .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1990, 2 (51) :10227-10234
[16]   VIBRATION EIGENMODES AND SIZE OF MICROCRYSTALLITES IN GLASS - OBSERVATION BY VERY-LOW-FREQUENCY RAMAN-SCATTERING [J].
DUVAL, E ;
BOUKENTER, A ;
CHAMPAGNON, B .
PHYSICAL REVIEW LETTERS, 1986, 56 (19) :2052-2055
[17]   THE ORIGIN OF THE 1ST SHARP DIFFRACTION PEAK IN THE STRUCTURE FACTOR OF COVALENT GLASSES AND LIQUIDS [J].
ELLIOTT, SR .
JOURNAL OF PHYSICS-CONDENSED MATTER, 1992, 4 (38) :7661-7678
[18]   A UNIFIED MODEL FOR THE LOW-ENERGY VIBRATIONAL BEHAVIOR OF AMORPHOUS SOLIDS [J].
ELLIOTT, SR .
EUROPHYSICS LETTERS, 1992, 19 (03) :201-206
[20]   OBSERVATION OF A DYNAMIC ANOMALY IN THE LIQUID-GLASS TRANSFORMATION RANGE BY BRILLOUIN-SCATTERING [J].
ELMROTH, M ;
BORJESSON, L ;
TORELL, LM .
PHYSICAL REVIEW LETTERS, 1992, 68 (01) :79-82