共 23 条
Measurements of methane emissions at natural gas production sites in the United States
被引:398
作者:
Allen, David T.
[1
]
Torres, Vincent M.
[1
]
Thomas, James
[1
]
Sullivan, David W.
[1
]
Harrison, Matthew
[2
]
Hendler, Al
[2
]
Herndon, Scott C.
[3
]
Kolb, Charles E.
[3
]
Fraser, Matthew P.
[4
]
Hill, A. Daniel
[5
]
Lamb, Brian K.
[6
]
Miskimins, Jennifer
[7
]
Sawyer, Robert F.
[8
]
Seinfeld, John H.
[9
]
机构:
[1] Univ Texas Austin, Ctr Energy & Environm Resources, Austin, TX 78758 USA
[2] URS Corp, Austin, TX 78729 USA
[3] Aerodyne Res Inc, Billerica, MA 01821 USA
[4] Arizona State Univ, Sch Sustainable Engn & Built Environm, Tempe, AZ 85287 USA
[5] Texas A&M Univ, Dept Petr Engn, College Stn, TX 77843 USA
[6] Washington State Univ, Dept Civil & Environm Engn, Pullman, WA 99164 USA
[7] Colorado Sch Mines, Dept Petr Engn, Golden, CO 80401 USA
[8] Univ Calif Berkeley, Dept Mech Engn, Berkeley, CA 94720 USA
[9] CALTECH, Dept Chem Engn, Pasadena, CA 91125 USA
来源:
关键词:
greenhouse gas emissions;
hydraulic fracturing;
TRACER METHODS;
SHALE GAS;
LEAKAGE;
RESOURCES;
IMPACTS;
COAL;
D O I:
10.1073/pnas.1304880110
中图分类号:
O [数理科学和化学];
P [天文学、地球科学];
Q [生物科学];
N [自然科学总论];
学科分类号:
07 ;
0710 ;
09 ;
摘要:
Engineering estimates of methane emissions from natural gas production have led to varied projections of national emissions. This work reports direct measurements of methane emissions at 190 onshore natural gas sites in the United States (150 production sites, 27 well completion flowbacks, 9 well unloadings, and 4 workovers). For well completion flowbacks, which clear fractured wells of liquid to allow gas production, methane emissions ranged from 0.01 Mg to 17 Mg (mean = 1.7 Mg; 95% confidence bounds of 0.67-3.3 Mg), compared with an average of 81 Mg per event in the 2011 EPA national emission inventory from April 2013. Emission factors for pneumatic pumps and controllers as well as equipment leaks were both comparable to and higher than estimates in the national inventory. Overall, if emission factors from this work for completion flowbacks, equipment leaks, and pneumatic pumps and controllers are assumed to be representative of national populations and are used to estimate national emissions, total annual emissions from these source categories are calculated to be 957 Gg of methane (with sampling and measurement uncertainties estimated at +/- 200 Gg). The estimate for comparable source categories in the EPA national inventory is similar to 1,200 Gg. Additional measurements of unloadings and workovers are needed to produce national emission estimates for these source categories. The 957 Gg in emissions for completion flowbacks, pneumatics, and equipment leaks, coupled with EPA national inventory estimates for other categories, leads to an estimated 2,300 Gg of methane emissions from natural gas production (0.42% of gross gas production).
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页码:17768 / 17773
页数:6
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