Nanostructured Electrodes for High-Performance Pseudocapacitors

被引:521
作者
Lu, Qi [1 ]
Chen, Jingguang G. [2 ]
Xiao, John Q. [3 ]
机构
[1] Univ Delaware, Dept Chem & Biomol Engn, Newark, DE 19716 USA
[2] Columbia Univ, Dept Chem Engn, New York, NY 10027 USA
[3] Univ Delaware, Dept Phys & Astron, Newark, DE 19716 USA
基金
美国国家科学基金会;
关键词
electrodes; metal oxides; nanomaterials; pseudocapacitors; supercapacitors; PORE-SIZE; SUPERCAPACITOR ELECTRODES; ELECTROCHEMICAL STORAGE; CARBON NANOTUBES; NICKEL-HYDROXIDE; ENERGY-STORAGE; OXIDE; CAPACITANCE; GRAPHENE/MNO2; RESISTANCE;
D O I
10.1002/anie.201203201
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The depletion of traditional energy resources as well as the desire to reduce high CO2 emissions associated with energy production means that energy storage is now becoming more important than ever. New functional electrode materials are urgently needed for next-generation energy storage systems, such as supercapacitors or batteries, to meet the ever increasing demand for higher energy and power densities. Advances in nanotechnology are essential to meet those future challenges. It is critical to develop ways of synthesizing new nanomaterials with enhanced properties or combinations of properties to meet future challenges. In this Minireview we discuss several important recent studies in developing nanostructured pseudocapacitor electrodes, and summarize three major parameters that are the most important in determining the performance of electrode materials. A technique to optimize these parameters simultaneously and to achieve both high energy and power densities is also introduced.
引用
收藏
页码:1882 / 1889
页数:8
相关论文
共 59 条
[1]   Effect of O2 flow concentration during reactive sputtering of Ni oxide thin films on their electrochemical and electrochromic properties in aqueous acidic and basic electrolyte solutions [J].
Abe, Yoshio ;
Lee, Se-Hee ;
Zayim, Esra Ozkan ;
Tracy, C. Edwin ;
Pitts, J. Roland ;
Deb, Satyen K. .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS, 2006, 45 (10A) :7780-7783
[2]  
[Anonymous], ANGEW CHEM INT ED
[3]   Nanostructured materials for advanced energy conversion and storage devices [J].
Aricò, AS ;
Bruce, P ;
Scrosati, B ;
Tarascon, JM ;
Van Schalkwijk, W .
NATURE MATERIALS, 2005, 4 (05) :366-377
[4]  
Brezesinski T, 2010, NAT MATER, V9, P146, DOI [10.1038/NMAT2612, 10.1038/nmat2612]
[5]  
Bruce P.G., 2008, Angew. Chem, V120, P2972
[6]   Nanomaterials for rechargeable lithium batteries [J].
Bruce, Peter G. ;
Scrosati, Bruno ;
Tarascon, Jean-Marie .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (16) :2930-2946
[7]  
Chmiola J, 2006, SCIENCE, V313, P1760, DOI 10.1126/science/1132195
[8]  
Chmiola J., 2008, ANGEW CHEM INT EDIT, V120, P3440, DOI DOI 10.1002/ANGE.200704894
[9]   Desolvation of ions in subnanometer pores and its effect on capacitance and double-layer theory [J].
Chmiola, John ;
Largeot, Celine ;
Taberna, Pierre-Louis ;
Simon, Patrice ;
Gogotsi, Yury .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2008, 47 (18) :3392-3395
[10]   Monolithic Carbide-Derived Carbon Films for Micro-Supercapacitors [J].
Chmiola, John ;
Largeot, Celine ;
Taberna, Pierre-Louis ;
Simon, Patrice ;
Gogotsi, Yury .
SCIENCE, 2010, 328 (5977) :480-483