Radiative forcing from household fuel burning in Asia

被引:26
作者
Aunan, Kristin [1 ]
Berntsen, Terje K. [1 ,2 ]
Myhre, Gunnar [1 ,2 ]
Rypdal, Kristin [1 ]
Streets, David G. [3 ]
Woo, Jung-Hun [4 ]
Smith, Kirk R. [5 ]
机构
[1] CICERO, N-0318 Oslo, Norway
[2] Univ Oslo, Dept Geosci, N-0315 Oslo, Norway
[3] Argonne Natl Lab, Decis & Informat Sci Div, Argonne, IL 60439 USA
[4] Konkuk Univ, Dept Adv Technol Fus, Seoul 143701, South Korea
[5] Univ Calif Berkeley, Sch Publ Hlth, Berkeley, CA 94720 USA
关键词
Solid fuel burning; Asia; Emissions; Radiative forcing; Air pollutants; GLOBAL AEROSOL; AIR-POLLUTION; EMISSIONS; CLIMATE; TRANSPORT; GASES; REDUCTIONS; MODEL;
D O I
10.1016/j.atmosenv.2009.07.053
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Household fuel use in developing countries, particularly as biomass and coal, is a major source of carbonaceous aerosols and other air pollutants affecting health and climate. Using state-of-the-art emission inventories, a global three-dimensional photochemical tracer/transport model of the troposphere, and a global radiative transfer model based on methods presented in the latest IPCC Assessment Report (2007-AR4), we estimate the radiative forcing (RF) attributable to household fuel combustion in Asia in terms of current global annual-mean RF and future global integrated RF for a one-year pulse of emissions (2000) over two time horizons (100 and 20 years). Despite the significant emissions of black carbon (BC) aerosols, these estimates indicate that shorter-lived (non-Kyoto) air pollutants from household fuel use in the region overall seem to exert a small net negative RF because of the strong influence of reflective aerosols. There are, however, major uncertainties in emission estimates for solid fuel burning, and about the sustainability of household fuel wood harvesting in Asia (the carbon neutrality of harvesting). In addition, there is still substantial uncertainty associated with the BC radiative forcing. As a result we find that the sign of the RF from household biomass burning in the region cannot be established. While recognizing the value of integrating climate change and air pollution policies, we are concerned that for a 'Kyoto style' post-Kyoto treaty (with global cap-and-trade and the Global Warming Potential as the metric) expanding the basket of components with a selection of short-lived species without also including the wider range of co-emitted species may lead to unintended consequences for global-scale climate. Additional measurement, modelling, and policy research is urgently needed to reduce the uncertainties so that the net impact on climate of emissions and mitigation measures in this sector can be accurately assessed. (C) 2009 Elsevier Ltd. All rights reserved.
引用
收藏
页码:5674 / 5681
页数:8
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