Excitons in carbon nanotubes with broken time-reversal symmetry

被引:96
作者
Zaric, S
Ostojic, GN
Shaver, J
Kono, J [1 ]
Portugall, O
Frings, PH
Rikken, GLJA
Furis, M
Crooker, SA
Wei, X
Moore, VC
Hauge, RH
Smalley, RE
机构
[1] Rice Univ, Dept Elect & Comp Engn, Houston, TX 77005 USA
[2] Lab Natl Champs Magnet Pulses, F-31432 Toulouse 04, France
[3] Los Alamos Natl Lab, Natl High Magnet Field Lab, Los Alamos, NM 87545 USA
[4] Florida State Univ, Natl High Magnet Field Lab, Tallahassee, FL 32310 USA
[5] Rice Univ, Dept Chem, Houston, TX 77005 USA
基金
美国国家科学基金会;
关键词
D O I
10.1103/PhysRevLett.96.016406
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Near-infrared magneto-optical spectroscopy of single-walled carbon nanotubes reveals two absorption peaks with an equal strength at high magnetic fields (> 55 T). We show that the peak separation is determined by the Aharonov-Bohm phase due to the tube-threading magnetic flux, which breaks the time-reversal symmetry and lifts the valley degeneracy. This field-induced symmetry breaking thus overcomes the Coulomb-induced intervalley mixing which is predicted to make the lowest exciton state optically inactive (or dark).
引用
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页数:4
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共 27 条
[11]   Ratio problem in single carbon nanotube fluorescence spectroscopy [J].
Kane, CL ;
Mele, EJ .
PHYSICAL REVIEW LETTERS, 2003, 90 (20) :4
[12]   Exciton binding energies in carbon nanotubes from two-photon photoluminescence [J].
Maultzsch, J ;
Pomraenke, R ;
Reich, S ;
Chang, E ;
Prezzi, D ;
Ruini, A ;
Molinari, E ;
Strano, MS ;
Thomsen, C ;
Lienau, C .
PHYSICAL REVIEW B, 2005, 72 (24)
[13]   Band gap fluorescence from individual single-walled carbon nanotubes [J].
O'Connell, MJ ;
Bachilo, SM ;
Huffman, CB ;
Moore, VC ;
Strano, MS ;
Haroz, EH ;
Rialon, KL ;
Boul, PJ ;
Noon, WH ;
Kittrell, C ;
Ma, JP ;
Hauge, RH ;
Weisman, RB ;
Smalley, RE .
SCIENCE, 2002, 297 (5581) :593-596
[14]   Stability of high-density one-dimensional excitons in carbon nanotubes under high laser excitation [J].
Ostojic, GN ;
Zaric, S ;
Kono, J ;
Moore, VC ;
Hauge, RH ;
Smalley, RE .
PHYSICAL REVIEW LETTERS, 2005, 94 (09)
[15]   Interband recombination dynamics in resonantly excited single-walled carbon nanotubes [J].
Ostojic, GN ;
Zaric, S ;
Kono, J ;
Strano, MS ;
Moore, VC ;
Hauge, RH ;
Smalley, RE .
PHYSICAL REVIEW LETTERS, 2004, 92 (11) :117402-1
[16]   Exciton effects in carbon nanotubes [J].
Pedersen, TG .
CARBON, 2004, 42 (5-6) :1007-1010
[17]   Radiative lifetime of excitons in carbon nanotubes [J].
Perebeinos, V ;
Tersoff, J ;
Avouris, P .
NANO LETTERS, 2005, 5 (12) :2495-2499
[18]   Scaling of excitons in carbon nanotubes [J].
Perebeinos, V ;
Tersoff, J ;
Avouris, P .
PHYSICAL REVIEW LETTERS, 2004, 92 (25) :257402-1
[19]   Aharonov-Bohm spectral features and coherence lengths in carbon nanotubes [J].
Roche, S ;
Dresselhaus, G ;
Dresselhaus, MS ;
Saito, R .
PHYSICAL REVIEW B, 2000, 62 (23) :16092-16099
[20]   Magnetoelectronic and optical properties of carbon nanotubes [J].
Shyu, FL ;
Chang, CP ;
Chen, RB ;
Chiu, CW ;
Lin, MF .
PHYSICAL REVIEW B, 2003, 67 (04)