High-order harmonic generation in molecular gases

被引:80
作者
Lynga, C
LHuillier, A
Wahlstrom, CG
机构
[1] Department of Physics, Lund Institute of Technology
关键词
D O I
10.1088/0953-4075/29/14/032
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We present an experimental study of harmonic generation in molecular gases, using the fundamental (800 nm) and the second harmonic (400 nm) of a 150 fs titanium-sapphire laser at an intensity of similar to 2 x 10(14) W cm(-2). We compare the conversion efficiency and the maximum energy obtained in different species: rare gases (Ar, Xe), diatomic molecules (N-2, H-2, O-2, CO) and polyatomic molecules (SF6, N2O, CO2, CH4, C3H8). The harmonic spectra from molecular gases are very similar to those obtained in the atomic gases, with a plateau and a cutoff whose location is strongly correlated to the value of the ionization potential. The conversion efficiency is not higher than that of the rare gases.
引用
收藏
页码:3293 / 3302
页数:10
相关论文
共 28 条
[11]   HIGH-ORDER HARMONIC-GENERATION FROM ATOMS AND IONS IN THE HIGH-INTENSITY REGIME [J].
KRAUSE, JL ;
SCHAFER, KJ ;
KULANDER, KC .
PHYSICAL REVIEW LETTERS, 1992, 68 (24) :3535-3538
[12]  
KULANDER KC, 1993, NATO ADV SCI INST SE, V316, P95, DOI 10.1007/978-1-4615-7963-2_10
[13]   2-COLOR TIME-RESOLVED SPECTROSCOPY OF HELIUM USING HIGH-ORDER HARMONICS [J].
LARSSON, J ;
MEVEL, E ;
ZERNE, R ;
LHUILLIER, A ;
WAHLSTROM, CG ;
SVANBERG, S .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1995, 28 (03) :L53-L58
[14]  
LEWENSTEIN M, COMMUNICATION
[15]   HIGH-ORDER HARMONIC-GENERATION IN RARE-GASES WITH A 1-PS 1053-NM LASER [J].
LHUILLIER, A ;
BALCOU, P .
PHYSICAL REVIEW LETTERS, 1993, 70 (06) :774-777
[16]   HIGH-ORDER HARMONICS - A COHERENT SOURCE IN THE XUV RANGE [J].
LHUILLIER, A ;
AUGUSTE, T ;
BALCOU, PH ;
CARRE, B ;
MONOT, P ;
SALIERES, P ;
ALTUCCI, C ;
GAARDE, MB ;
LARSSON, J ;
MEVEL, E ;
STARCZEWSKI, T ;
SVANBERG, S ;
WAHLSTROM, CG ;
ZERNE, R ;
BUDIL, KS ;
DITMIRE, T ;
PERRY, MD .
JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS, 1995, 4 (03) :647-665
[17]   HIGH-ORDER HARMONIC-GENERATION CUTOFF [J].
LHUILLIER, A ;
LEWENSTEIN, M ;
SALIERES, P ;
BALCOU, P ;
IVANOV, MY ;
LARSSON, J ;
WAHLSTROM, CG .
PHYSICAL REVIEW A, 1993, 48 (05) :R3433-R3436
[18]   HIGH HARMONIC-GENERATION IN ATOMIC AND DIATOMIC MOLECULAR GASES USING INTENSE PICOSECOND LASER-PULSES - A COMPARISON [J].
LIANG, Y ;
AUGST, S ;
CHIN, SL ;
BEAUDOIN, Y ;
CHAKER, M .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1994, 27 (20) :5119-5130
[19]   HIGH-ORDER HARMONIC-GENERATION USING INTENSE FEMTOSECOND PULSES [J].
MACKLIN, JJ ;
KMETEC, JD ;
GORDON, CL .
PHYSICAL REVIEW LETTERS, 1993, 70 (06) :766-769
[20]   HARMONIC-GENERATION IN MOLECULAR-SYSTEMS - APPLICATION TO H-2(+) IN INTENSE LASER FIELDS [J].
MOISEYEV, N ;
CHRYSOS, M ;
ATABEK, O ;
LEFEBVRE, R .
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS, 1995, 28 (10) :2007-2020