Quasi-one-dimensional S=1/2 magnet Pb[Cu(SO4)(OH)2]:: frustration due to competing in-chain exchange

被引:23
作者
Baran, M
Jedrzejczak, A
Szymczak, H
Maltsev, V
Kamieniarz, G [3 ]
Szukowski, G
Loison, C
Ormeci, A
Drechsler, SL
Rosner, H
机构
[1] Polish Acad Sci, Inst Phys, PL-02668 Warsaw, Poland
[2] Moscow MV Lomonosov State Univ, Dept Geol, Moscow 119899, Russia
[3] Adam Mickiewicz Univ, Inst Phys, Ul Umultowska 85, PL-61614 Poznan, Poland
[4] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany
[5] Max Planck Inst Chem Phys Fester Stoffe, D-01187 Dresden, Germany
[6] IFW Dresden, Inst Festkorpertheorie, D-01171 Dresden, Germany
来源
PHYSICA STATUS SOLIDI C - CURRENT TOPICS IN SOLID STATE PHYSICS, VOL 3, NO1 | 2006年 / 3卷 / 01期
关键词
D O I
10.1002/pssc.200562523
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Zero-field susceptibility and specific heat of Pb[CU(SO4)(OH)(2)] (linarite) single crystal were measured. In order to verify that linarite is a quasi-one-dimensional system with competing nearest-neighbour and next-nearest-neighbour in-chain exchange interaction (J(1) approximate to -30 K, J(2) approximate to 15 K), theoretical results based on electronic structure calculations within the LDA and a phenomenological modelling using the finite-temperature transfer-matrix method are taken into account. The possibility of various ground states is discussed in terms of the screened onsite repulsion Us: commensurate Neel or spin-Peierls phases versus incommensurate spiral states with acute or obtuse pitch angles.
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收藏
页码:220 / +
页数:3
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