Srm-3Bi4TimO3m+3 (m = 4, 5, 6) thin films were grown on (100)MgO and (100)Pt/(100)MgO substrates by the pulsed laser deposition (PLD) method. X-ray diffraction (XRD) revealed c-axis-oriented crystal growth of each Srm-3Bi4TimO3m+3 film. Reflection high-energy electron diffraction (RHEED) from the films showed a streak pattern which indicates the epitaxial ordering of the fabricated thin films. Fundamental optical absorption of SrBi4Ti4O15, Sr2Bi4Ti5O18 and Sr3Bi4Ti6O21 films started at 3.4, 3.5 and 3.7 eV, respectively. Moreover, the Fourier transform infrared (FTIR) spectra also revealed a systematic change in their LO-phonon absorption dip structure.