Low Driving Voltage and High Mobility Ambipolar Field-Effect Transistors with PbS Colloidal Nanocrystals

被引:106
作者
Bisri, Satria Zulkarnaen [1 ]
Piliego, Claudia [1 ]
Yarema, Maksym [2 ]
Heiss, Wolfgang [2 ]
Loi, Maria Antonietta [1 ]
机构
[1] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands
[2] Univ Linz, Inst Semicond & Solid State Phys, A-4040 Linz, Austria
基金
欧洲研究理事会;
关键词
colloidal nanocrystals; ambipolar transistor; layer-by-layer assembly; electrolyte gating; metal chalcogenides; QUANTUM-DOT SOLIDS; N-CHANNEL; PHOTOVOLTAICS; LAYERS;
D O I
10.1002/adma.201205041
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
PbS colloidal nanocrystals (NCs) are promising materials for optoelectronic devices, due to their size-tunable properties. However, there is still minimal understanding of their charge transport mechanism. Through a combination of ligand selections, ambipolar transistor structure optimization, and electrochemical gating usage, high carrier mobility is achieved. The outstanding device characteristics open possibility to investigate the intrinsic transport properties of PbS NCs. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:4309 / 4314
页数:6
相关论文
共 37 条
[1]   Organic Single-Crystal Light-Emitting Transistor Coupling with Optical Feedback Resonators [J].
Bisri, Satria Zulkarnaen ;
Sawabe, Kosuke ;
Imakawa, Masaki ;
Maruyama, Kenichi ;
Yamao, Takeshi ;
Hotta, Shu ;
Iwasa, Yoshihiro ;
Takenobu, Taishi .
SCIENTIFIC REPORTS, 2012, 2
[2]   p-i-n Homojunction in Organic Light-Emitting Transistors [J].
Bisri, Satria Zulkarnaen ;
Takenobu, Taishi ;
Sawabe, Kosuke ;
Tsuda, Satoshi ;
Yomogidao, Yohei ;
Yamao, Takeshi ;
Hotta, Shu ;
Adachi, Chihaya ;
Iwasa, Yoshihiro .
ADVANCED MATERIALS, 2011, 23 (24) :2753-2758
[3]   Electron transport in rubrene single-crystal transistors [J].
Bisri, Satria Zulkarnaen ;
Takenobu, Taishi ;
Takahashi, Tetsuo ;
Iwasa, Yoshihiro .
APPLIED PHYSICS LETTERS, 2010, 96 (18)
[4]   Bandlike Transport in Strongly Coupled and Doped Quantum Dot Solids: A Route to High-Performance Thin-Film Electronics [J].
Choi, Ji-Hyuk ;
Fafarman, Aaron T. ;
Oh, Soong Ju ;
Ko, Dong-Kyun ;
Kim, David K. ;
Diroll, Benjamin T. ;
Muramoto, Shin ;
Gillen, J. Greg ;
Murray, Christopher B. ;
Kagan, Cherie R. .
NANO LETTERS, 2012, 12 (05) :2631-2638
[5]   Photogenerated Exciton Dissociation in Highly Coupled Lead Salt Nanocrystal Assemblies [J].
Choi, Joshua J. ;
Luria, Justin ;
Hyun, Byung-Ryool ;
Bartnik, Adam C. ;
Sun, Liangfeng ;
Lim, Yee-Fun ;
Marohn, John A. ;
Wise, Frank W. ;
Hanrath, Tobias .
NANO LETTERS, 2010, 10 (05) :1805-1811
[6]   From Monolayer to Multilayer N-Channel Polymeric Field-Effect Transistors with Precise Conformational Order [J].
Fabiano, Simone ;
Musumeci, Chiara ;
Chen, Zhihua ;
Scandurra, Antonino ;
Wang, He ;
Loo, Yueh-Lin ;
Facchetti, Antonio ;
Pignataro, Bruno .
ADVANCED MATERIALS, 2012, 24 (07) :951-+
[7]  
Hwang HY, 2012, NAT MATER, V11, P103, DOI [10.1038/nmat3223, 10.1038/NMAT3223]
[8]  
Ip AH, 2012, NAT NANOTECHNOL, V7, P577, DOI [10.1038/NNANO.2012.127, 10.1038/nnano.2012.127]
[9]   Enhanced Mobility-Lifetime Products in PbS Colloidal Quantum Dot Photovoltaics [J].
Jeong, Kwang S. ;
Tang, Jiang ;
Liu, Huan ;
Kim, Jihye ;
Schaefer, Andrew W. ;
Kemp, Kyle ;
Levina, Larissa ;
Wang, Xihua ;
Hoogland, Sjoerd ;
Debnath, Ratan ;
Brzozowski, Lukasz ;
Sargent, Edward H. ;
Asbury, John B. .
ACS NANO, 2012, 6 (01) :89-99
[10]   High Carrier Densities Achieved at Low Voltages in Ambipolar PbSe Nanocrystal Thin-Film Transistors [J].
Kang, Moon Sung ;
Lee, Jiyoul ;
Norris, David J. ;
Frisbie, C. Daniel .
NANO LETTERS, 2009, 9 (11) :3848-3852