Effect of rising Asian emissions on surface ozone in the United States

被引:336
作者
Jacob, DJ
Logan, JA
Murti, PP
机构
[1] Harvard Univ, Div Engn & Appl Sci, Cambridge, MA 02138 USA
[2] Harvard Univ, Dept Earth & Planetary Sci, Cambridge, MA 02138 USA
关键词
D O I
10.1029/1999GL900450
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
The effect of increasing fossil fuel combustion in eastern Asia on surface O-3 air pollution in the United States is examined with a global three-dimensional tropospheric chemistry model. Tripling of Asian anthropogenic emissions from 1985 to 2010 is expected to increase monthly mean O-3 concentrations by 2-6 ppbv in the western United States and by 1-3 ppbv in the eastern United States, the maximum effect being in April-June. This increase would more than offset the benefits of 25% domestic reductions in anthropogenic emissions of NOx and hydrocarbons in the western United States. Asian influence may be less under the stagnant conditions leading to violations of the U.S. air quality standard. Nevertheless, our results suggest that a global perspective is necessary when designing a strategy to meet regional O-3 air quality objectives.
引用
收藏
页码:2175 / 2178
页数:4
相关论文
共 28 条
[21]   EVIDENCE OF A LONG-TERM INCREASE IN TROPOSPHERIC OZONE FROM PIC DU MIDI DATA SERIES - CONSEQUENCES - POSITIVE RADIATIVE FORCING [J].
MARENCO, A ;
GOUGET, H ;
NEDELEC, P ;
PAGES, JP ;
KARCHER, F .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1994, 99 (D8) :16617-16632
[22]   A STUDY OF THE DEPENDENCE OF RURAL OZONE ON OZONE PRECURSORS IN THE EASTERN UNITED-STATES [J].
MCKEEN, SA ;
HSIE, EY ;
LIU, SC .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1991, 96 (D8) :15377-15394
[23]  
MERRILL JT, 1989, CHEM OCEANOGR, V10, P15
[24]   A GLOBAL INVENTORY OF VOLATILE ORGANIC-COMPOUND EMISSIONS FROM ANTHROPOGENIC SOURCES [J].
PICCOT, SD ;
WATSON, JJ ;
JONES, JW .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1992, 97 (D9) :9897-9912
[25]  
SAVOIE DL, 1989, CHEM OCEANOGR, V10, P220
[26]   Implications of the new ozone National Ambient Air Quality Standards for compliance in rural areas [J].
Saylor, RD ;
Chameides, WL ;
Cowling, EB .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1998, 103 (D23) :31137-31141
[27]   THE SENSITIVITY OF OZONE TO NITROGEN-OXIDES AND HYDROCARBONS IN REGIONAL OZONE EPISODES [J].
SILLMAN, S ;
LOGAN, JA ;
WOFSY, SC .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1990, 95 (D2) :1837-1851
[28]   Global simulation of tropospheric O3-NOx-hydrocarbon chemistry 2.: Model evaluation and global ozone budget [J].
Wang, YH ;
Logan, JA ;
Jacob, DJ .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1998, 103 (D9) :10727-10755