Air-steam gasification of biomass in a fluidized bed under simulated autothermal and adiabatic conditions

被引:73
作者
Campoy, Manuel [1 ]
Gomez-Barea, Alberto [1 ]
Villanueva, Angel L. [1 ]
Ollero, Pedro [1 ]
机构
[1] Univ Seville, Escuela Super Ingn, Chem & Environm Engn Dept, Bioenergy Grp, Seville 41092, Spain
关键词
D O I
10.1021/ie800220t
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
Biomass gasification tests with air-steam mixtures were conducted in a bubbling fluidized-bed (FB) gasification pilot plant. The effect of steam addition on the performance of gasification was studied for different air-to-biomass ratios and biomass throughputs. The reactor was operated near adiabatic conditions, with the aim of reproducing the behavior of full-scale FB units. The temperature of the air-steam mixture was fixed at 400 'C for all tests, a value that can be achieved by energy recovery from the off-gas without tar-condensing problems. The stoichiometric ratio (ratio of actual to stoichiometric air flow rates) and steam-to-biomass flow rate ratio were varied from 0.19 to 0.35 and from 0 to 0.45, respectively. It is shown that the proper selection of operating conditions makes it possible to increase the gasification efficiency from 40% to 60%, while maintaining the low heating value of the gas at around 5 MJ/Nm(3). In addition, an appreciable increase of char and tar conversion is achieved. The air-steam gasification concept explored in this work is an interesting option for the improvement of direct air-blown biomass gasification because it can improve the process efficiency considerably without significantly increasing capital costs.
引用
收藏
页码:5957 / 5965
页数:9
相关论文
共 26 条
[1]   Modeling circulating fluidized bed biomass gasifiers. A pseudo-rigorous model for stationary state [J].
Corella, J ;
Sanz, A .
FUEL PROCESSING TECHNOLOGY, 2005, 86 (09) :1021-1053
[2]   Study about the kinetic processes of biomass steam gasification [J].
Dupont, Capucine ;
Boissonnet, Guillaume ;
Seller, Jean-Marie ;
Gauthier, Paola ;
Schweich, Daniel .
FUEL, 2007, 86 (1-2) :32-40
[3]   The study of reactions influencing the biomass steam gasification process [J].
Franco, C ;
Pinto, F ;
Gulyurtlu, I ;
Cabrita, I .
FUEL, 2003, 82 (07) :835-842
[4]   Biomass gasification in atmospheric and bubbling fluidized bed: Effect of the type of gasifying agent on the product distribution [J].
Gil, J ;
Corella, J ;
Aznar, MP ;
Caballero, MA .
BIOMASS & BIOENERGY, 1999, 17 (05) :389-403
[5]   Pilot-plant gasification of olive stone:: a technical assessment [J].
Gómez-Barea, A ;
Arjona, R ;
Ollero, P .
ENERGY & FUELS, 2005, 19 (02) :598-605
[6]  
GOMEZBAREA A, 2005, P 19 INT C FLUID BED
[7]  
GOMEZBAREA A, DEVOLATILISATI UNPUB
[8]  
GOOD J, 2005, CEN BT TF 143 ORGANI
[9]   STEAM GASIFICATION OF LIGNOCELLULOSIC RESIDUES IN A FLUIDIZED-BED AT A SMALL PILOT SCALE - EFFECT OF THE TYPE OF FEEDSTOCK [J].
HERGUIDO, J ;
CORELLA, J ;
GONZALEZSAIZ, J .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 1992, 31 (05) :1274-1282
[10]   Thermodynamic limits and actual product yields and compositions in Biomass gasification processes [J].
Jand, N ;
Brandani, V ;
Foscolo, PU .
INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH, 2006, 45 (02) :834-843