Nitrogen-Doped Colloidal Graphene Quantum Dots and Their Size-Dependent Electrocatalytic Activity for the Oxygen Reduction Reaction

被引:529
作者
Li, Qiqi [1 ]
Zhang, Sheng [2 ]
Dai, Liming [2 ]
Li, Liang-shi [1 ]
机构
[1] Indiana Univ, Dept Chem, Bloomington, IN 47405 USA
[2] Case Western Reserve Univ, Dept Macromol Sci & Engn, Cleveland, OH 44106 USA
基金
美国国家科学基金会;
关键词
CATALYSTS; ARRAYS;
D O I
10.1021/ja309270h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Nitrogen doping has been a powerful way to modify the properties of carbon materials ranging from activated carbon to graphene. Here we report on a solution chemistry approach to nitrogen-doped colloidal graphene quantum dots with well-defined structures. N-doping was demonstrated to significantly affect the properties of the quantum dots, including the emergence of size-dependent electrocatalytic activity for the oxygen reduction reaction.
引用
收藏
页码:18932 / 18935
页数:4
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