What is the effect of cloud inhomogeneities on actinic fluxes and chemical species concentrations?

被引:5
作者
Bouet, C [1 ]
Szczap, F [1 ]
Leriche, M [1 ]
Benassi, A [1 ]
机构
[1] Univ Clermont Ferrand, Ctr Natl Rech Sci, Lab Meteorol Phys, Aubiere, France
关键词
D O I
10.1029/2005GL024727
中图分类号
P [天文学、地球科学];
学科分类号
07 ;
摘要
The purpose of the present paper is to evaluate the bias introduced by the commonly used homogeneous plane-parallel cloud hypothesis in the computation of actinic fluxes, photolysis coefficients, and main tropospheric species concentrations. Accordingly, these quantities obtained for an inhomogeneous cloud field generated with a stochastic model are compared to their homogeneous plane-parallel equivalent. Results show that neglecting cloud inhomogeneities has a significant impact on actinic flux. For instance, the bias introduced by the homogeneous plane-parallel cloud hypothesis can reach more than 100% below the cloud leading to a comparable bias in photolysis coefficients and, in turn, creating an enhancement of the oxidizing capacity of the system.
引用
收藏
页数:4
相关论文
共 41 条
[11]  
2
[12]   Comparison of observed and simulated NO2 photodissociation frequencies in a cloudless atmosphere and in continental boundary layer clouds [J].
Früh, B ;
Trautmann, T ;
Wendisch, M ;
Keil, A .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2000, 105 (D8) :9843-9857
[13]  
HARSHVARDHAN, 1982, J ATMOS SCI, V39, P1853, DOI 10.1175/1520-0469(1982)039<1853:TEOBOC>2.0.CO
[14]  
2
[15]  
JOSEPH JH, 1976, J ATMOS SCI, V33, P2452, DOI 10.1175/1520-0469(1976)033<2452:TDEAFR>2.0.CO
[16]  
2
[17]   Actinic radiation and photolysis processes in the lower troposphere:: Effect of clouds and aerosols [J].
Junkermann, W ;
Brühl, C ;
Perner, D ;
Eckstein, E ;
Trautmann, T ;
Früh, B ;
Dlugi, R ;
Gori, T ;
Ruggaber, A ;
Reuder, J ;
Zelger, M ;
Hofzumahaus, A ;
Kraus, A ;
Rohrer, F ;
Brüning, D ;
Moortgat, G ;
Horowitz, A ;
Tadic, J .
JOURNAL OF ATMOSPHERIC CHEMISTRY, 2002, 42 (01) :413-441
[18]   Solar actinic flux and photolysis frequency determinations by radiometers and a radiative transfer model at Rishiri Island: comparisons, cloud effects, and detection of an aerosol plume from Russian forest fires [J].
Kanaya, Y ;
Kajii, Y ;
Akimoto, H .
ATMOSPHERIC ENVIRONMENT, 2003, 37 (18) :2463-2475
[19]   Microphysical properties of continental clouds from in situ measurements [J].
Korolev, AV ;
Isaac, GA ;
Mazin, P ;
Barker, HW .
QUARTERLY JOURNAL OF THE ROYAL METEOROLOGICAL SOCIETY, 2001, 127 (576) :2117-2151
[20]   Nitrous acid and nitrite in the atmosphere [J].
Lammel, G ;
Cape, JN .
CHEMICAL SOCIETY REVIEWS, 1996, 25 (05) :361-+