Calculation of conductance spectra of silver clusters on graphite

被引:5
作者
De Menech, M
Saalmann, U
Garcia, ME
机构
[1] Max Planck Inst Phys Komplexer Syst, D-01187 Dresden, Germany
[2] Univ Kassel, Fachbereich Naturwissenschaft, D-34132 Kassel, Germany
来源
APPLIED PHYSICS A-MATERIALS SCIENCE & PROCESSING | 2006年 / 82卷 / 01期
关键词
D O I
10.1007/s00339-005-3346-6
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The transport properties of Ag-n clusters, 40 < n < 100, deposited on crystalline graphite and probed with a tunneling tip are analyzed by using non-equilibrium Green's functions. Current-voltage characteristics are computed accounting for self-consistent charge redistribution in the cluster caused by coupling to the surface and the external bias. The differential conductance is compared to the density of states of the supported clusters at equilibrium, highlighting the effects of charging and substrate properties on the measured spectrum.
引用
收藏
页码:113 / 116
页数:4
相关论文
共 19 条
[1]   Scanning tunneling spectroscopy on deposited platinum clusters [J].
Bettac, A ;
Koller, L ;
Rank, V ;
Meiwes-Broer, KH .
SURFACE SCIENCE, 1998, 402 (1-3) :475-479
[2]   Density-functional method for nonequilibrium electron transport -: art. no. 165401 [J].
Brandbyge, M ;
Mozos, JL ;
Ordejón, P ;
Taylor, J ;
Stokbro, K .
PHYSICAL REVIEW B, 2002, 65 (16) :1654011-16540117
[3]   Electron transport through heterocyclic molecule: ab initio molecular orbital theory [J].
Cheng, WW ;
Liao, XY ;
Chen, H ;
Note, R ;
Mizuseki, H ;
Kawazoe, Y .
PHYSICS LETTERS A, 2004, 326 (5-6) :412-416
[4]   The energy of Ag adatoms and dimers on graphite [J].
Duffy, DM ;
Blackman, JA .
SURFACE SCIENCE, 1998, 415 (03) :L1016-L1019
[5]   Self-consistent-charge density-functional tight-binding method for simulations of complex materials properties [J].
Elstner, M ;
Porezag, D ;
Jungnickel, G ;
Elsner, J ;
Haugk, M ;
Frauenheim, T ;
Suhai, S ;
Seifert, G .
PHYSICAL REVIEW B, 1998, 58 (11) :7260-7268
[6]   Palladium nanocrystals on Al2O3:: Structure and adhesion energy [J].
Hansen, KH ;
Worren, T ;
Stempel, S ;
Lægsgaard, E ;
Bäumer, M ;
Freund, HJ ;
Besenbacher, F ;
Stensgaard, I .
PHYSICAL REVIEW LETTERS, 1999, 83 (20) :4120-4123
[7]   Tunneling spectroscopy on silver clusters at T=5 K:: size dependence and spatial energy shifts [J].
Hövel, H ;
Grimm, B ;
Bödecker, M ;
Fieger, K ;
Reihl, B .
SURFACE SCIENCE, 2000, 463 (01) :L603-L608
[8]   Electrical transport through individual DNA molecules [J].
Li, XQ ;
Yan, YJ .
APPLIED PHYSICS LETTERS, 2001, 79 (14) :2190-2192
[9]   LANDAUER FORMULA FOR THE CURRENT THROUGH AN INTERACTING ELECTRON REGION [J].
MEIR, Y ;
WINGREEN, NS .
PHYSICAL REVIEW LETTERS, 1992, 68 (16) :2512-2515
[10]   O(N) real-space method for ab initio quantum transport calculations:: Application to carbon nanotube-metal contacts -: art. no. 245423 [J].
Nardelli, MB ;
Fattebert, JL ;
Bernholc, J .
PHYSICAL REVIEW B, 2001, 64 (24)