In-situ photoelectron spectroscopy with online activity measurement for catalysis research

被引：19

作者：

Chang, Rui ^{[1
,2
]}

Hong, Young Pyo ^{[1
]}

Axnanda, Stephanus ^{[1
]}

Mao, Baohua ^{[1
,3
]}

Jabeen, Naila ^{[1
,4
]}

Wang, Suidong ^{[3
]}

Tai, Renzhong ^{[2
]}

Liu, Zhi ^{[1
]}

机构：

[1] Univ Calif Berkeley, Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94720 USA

[2] Chinese Acad Sci, Shanghai Synchrotron Radiat Facil, Shanghai Inst Appl Phys, Shanghai 201203, Peoples R China

[3] Soochow Univ, Inst Funct Nano & Soft Mat Lab FUNSOM, Suzhou 215123, Jiangsu, Peoples R China

[4] NS & CD, Natl Ctr Phys, Islamabad 44000, Pakistan

来源：

CURRENT APPLIED PHYSICS | 2012年 / 12卷 / 05期

关键词：

Ambient pressure photoelectron spectroscopy; Catalysis; In-situ; SURFACE; CO; OXIDATION; SCIENCE;

D O I：

10.1016/j.cap.2012.03.014

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

We report Ambient pressure X-ray Photoelectron Spectroscopy Endstation with an integrated chemical analytical system that consists of a residual gas analyzer in the 2nd differential pumping stage and a new low-reactive sample holder heating assembly. This system has a linear response to the reaction chamber gas pressure. The sample heating assembly also has a low dark reaction rate up to 400 degrees C for H-2 and CO oxidation. We expect this chemical analytical system will expand our capabilities in conducting inoperando catalysis research. (C) 2012 Elsevier B.V. All rights reserved.

引用

页码：1292 / 1296

页数：5

共 21 条

[1] Soft X-ray microscopy and spectroscopy at the molecular environmental science beamline at the Advanced Light Source [J].

Bluhm, H ;

Andersson, K ;

Araki, T ;

Benzerara, K ;

Brown, GE ;

Dynes, JJ ;

Ghosal, S ;

Gilles, MK ;

Hansen, HC ;

Hemminger, JC ;

Hitchcock, AP ;

Ketteler, G ;

Kilcoyne, ALD ;

Kneedler, E ;

Lawrence, JR ;

Leppard, GG ;

Majzlan, J ;

Mun, BS ;

Myneni, SCB ;

Nilsson, A ;

Ogasawara, H ;

Ogletree, DF ;

Pecher, K ;

Salmeron, M ;

Shuh, DK ;

Tonner, B ;

Tyliszczak, T ;

Warwick, T ;

Yoon, TH .

JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2006, 150 (2-3) :86-104

[2] Photoelectron spectroscopy of surfaces under humid conditions [J].

Bluhm, Hendrik .

JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2010, 177 (2-3) :71-84

[3]

Butcher D.R., 2011, J AM CHEM SOC

[4] In-situ study of the catalytic oxidation of CO on a Pt(110) surface using ambient pressure X-ray photoelectron spectroscopy [J].

Chung, Jen-Yang ;

Aksoy, Funda ;

Grass, Michael E. ;

Kondoh, Hiroshi ;

Ross, Phil, Jr. ;

Liu, Zhi ;

Mun, Bongjin Simon .

SURFACE SCIENCE, 2009, 603 (05) :L35-L38

[5] In Situ Characterization of Ceria Oxidation States in High-Temperature Electrochemical Cells with Ambient Pressure XPS [J].

DeCaluwe, Steven C. ;

Grass, Michael E. ;

Zhang, Chunjuan ;

El Gabaly, Farid ;

Bluhm, Hendrik ;

Liu, Zhi ;

Jackson, Gregory S. ;

McDaniel, Anthony H. ;

McCarty, Kevin F. ;

Farrow, Roger L. ;

Linne, Mark A. ;

Hussain, Zahid ;

Eichhorn, Bryan W. .

JOURNAL OF PHYSICAL CHEMISTRY C, 2010, 114 (46) :19853-19861

[6] Measuring individual overpotentials in an operating solid-oxide electrochemical cell [J].

El Gabaly, Farid ;

Grass, Michael ;

McDaniel, Anthony H. ;

Farrow, Roger L. ;

Linne, Mark A. ;

Hussain, Zahid ;

Bluhm, Hendrik ;

Liu, Zhi ;

McCarty, Kevin F. .

PHYSICAL CHEMISTRY CHEMICAL PHYSICS, 2010, 12 (38) :12138-12145

[7] Effect of O2, CO, and NO on Surface Segregation in a Rh0.5Pd0.5 Bulk Crystal and Comparison to Rh0.5Pd0.5 Nanoparticles [J].

Grass, Michael E. ;

Park, Mita ;

Aksoy, Fonda ;

Zhang, Yawen ;

Kunz, Martin ;

Liu, Zhi ;

Mon, Bongjin S. .

LANGMUIR, 2010, 26 (21) :16362-16367

[8] New ambient pressure photoemission endstation at Advanced Light Source beamline 9.3.2 [J].

Grass, Michael E. ;

Karlsson, Patrik G. ;

Aksoy, Funda ;

Lundqvist, Mans ;

Wannberg, Bjorn ;

Mun, Bongjin S. ;

Hussain, Zahid ;

Liu, Zhi .

REVIEW OF SCIENTIFIC INSTRUMENTS, 2010, 81 (05)

[9] Adsorbate coverages and surface reactivity in methanol oxidation over Cu(110):: An in situ photoelectron spectroscopy study [J].

Gunther, S. ;

Zhou, L. ;

Havecker, M. ;

Knop-Gericke, A. ;

Kleimenov, E. ;

Schlogl, R. ;

Imbihl, R. .

JOURNAL OF CHEMICAL PHYSICS, 2006, 125 (11)

[10] Formation of hydroxyl and water layers on MgO films studied with ambient pressure XPS [J].

Newberg, John T. ;

Starr, David E. ;

Yamamoto, Susumu ;

Kaya, Sarp ;

Kendelewicz, Tom ;

Mysak, Erin R. ;

Porsgaard, Soeren ;

Salmeron, Miquel B. ;

Brown, Gordon E., Jr. ;

Nilsson, Anders ;

Bluhm, Hendrik .

SURFACE SCIENCE, 2011, 605 (1-2) :89-94

← 1 2 3 →