New ambient pressure photoemission endstation at Advanced Light Source beamline 9.3.2

被引:231
作者
Grass, Michael E. [1 ,2 ]
Karlsson, Patrik G. [3 ]
Aksoy, Funda [1 ,4 ]
Lundqvist, Mans [3 ]
Wannberg, Bjorn [3 ,5 ]
Mun, Bongjin S. [2 ]
Hussain, Zahid [1 ]
Liu, Zhi [1 ]
机构
[1] Lawrence Berkeley Natl Lab, Adv Light Source, Berkeley, CA 94709 USA
[2] Hanyang Univ ERICA, Dept Appl Phys, Gyeonggi Do 426791, South Korea
[3] VG Scienta, SE-75228 Uppsala, Sweden
[4] Cukurova Univ, Dept Phys, TR-01330 Adana, Turkey
[5] BW Particle Opt AB, SE-82222 Alfta, Sweden
关键词
photoelectron spectroscopy; RAY PHOTOELECTRON-SPECTROSCOPY; IN-SITU; CO OXIDATION; SURFACE; MICROSCOPY; NANOPARTICLES; INTERFACES; SCIENCE; SYSTEM; ESCA;
D O I
10.1063/1.3427218
中图分类号
TH7 [仪器、仪表];
学科分类号
0804 ; 080401 ; 081102 ;
摘要
During the past decade, the application of ambient pressure photoemission spectroscopy (APPES) has been recognized as an important in situ tool to study environmental and materials science, energy related science, and many other fields. Several APPES endstations are currently under planning or development at the USA and international light sources, which will lead to a rapid expansion of this technique. The present work describes the design and performance of a new APPES instrument at the Advanced Light Source beamline 9.3.2 at Lawrence Berkeley National Laboratory. This new instrument, Scienta R4000 HiPP, is a result of collaboration between Advanced Light Source and its industrial partner VG-Scienta. The R4000 HiPP provides superior electron transmission as well as spectromicroscopy modes with 16 mu m spatial resolution in one dimension and angle-resolved modes with simulated 0.5 degrees angular resolution at 24 degrees acceptance. Under maximum transmission mode, the electron detection efficiency is more than an order of magnitude better than the previous endstation at beamline 9.3.2. Herein we describe the design and performance of the system, which has been utilized to record spectra above 2 mbar. (C) 2010 American Institute of Physics. [doi: 10.1063/1.3427218]
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页数:7
相关论文
共 34 条
[1]   Synchrotron-based photoelectron microscopy [J].
Barinov, Alexei ;
Dudin, Pavel ;
Gregoratti, Luca ;
Locatelli, Andrea ;
Mentes, Tevfik Onur ;
Nino, Miquel Angel ;
Kiskinova, Maya .
NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION A-ACCELERATORS SPECTROMETERS DETECTORS AND ASSOCIATED EQUIPMENT, 2009, 601 (1-2) :195-202
[2]   Methanol oxidation on a copper catalyst investigated using in situ X-ray photoelectron spectroscopy [J].
Bluhm, H ;
Hävecker, M ;
Knop-Gericke, A ;
Kleimenov, E ;
Schlögl, R ;
Teschner, D ;
Bukhtiyarov, VI ;
Ogletree, DF ;
Salmeron, M .
JOURNAL OF PHYSICAL CHEMISTRY B, 2004, 108 (38) :14340-14347
[3]   In situ x-ray photoelectron spectroscopy studies of gas-solid interfaces at near-ambient conditions [J].
Bluhm, Hendrik ;
Haevecker, Michael ;
Knop-Gericke, Axel ;
Kiskinova, Maya ;
Schloegl, Robert ;
Salmeron, Miquel .
MRS BULLETIN, 2007, 32 (12) :1022-1030
[4]   Photoelectron spectroscopy of surfaces under humid conditions [J].
Bluhm, Hendrik .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2010, 177 (2-3) :71-84
[5]  
Bruche E, 1932, ANN PHYS-BERLIN, V15, P145
[6]   ESCA MICROSCOPY BEAMLINE AT ELETTRA [J].
CASALIS, L ;
JARK, W ;
KISKINOVA, M ;
LONZA, D ;
MELPIGNANO, P ;
MORRIS, D ;
ROSEL, R ;
SAVOIA, A ;
ABRAMI, A ;
FAVA, C ;
FURLAN, P ;
PUGLIESE, R ;
VIVODA, D ;
SANDRIN, G ;
WEI, FQ ;
CONTARINI, S ;
DEANGELIS, L ;
GARIAZZO, C ;
NATALETTI, P ;
MORRISON, GR .
REVIEW OF SCIENTIFIC INSTRUMENTS, 1995, 66 (10) :4870-4875
[7]   Secondary electron emission and fundamentals of charging mechanisms in XPS [J].
Cazaux, Jacques .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2010, 178 :357-372
[8]   In-situ study of the catalytic oxidation of CO on a Pt(110) surface using ambient pressure X-ray photoelectron spectroscopy [J].
Chung, Jen-Yang ;
Aksoy, Funda ;
Grass, Michael E. ;
Kondoh, Hiroshi ;
Ross, Phil, Jr. ;
Liu, Zhi ;
Mun, Bongjin Simon .
SURFACE SCIENCE, 2009, 603 (05) :L35-L38
[9]   Angle-resolved photoemission studies of the cuprate superconductors [J].
Damascelli, A ;
Hussain, Z ;
Shen, ZX .
REVIEWS OF MODERN PHYSICS, 2003, 75 (02) :473-541
[10]  
FENG J, 2008, SCI MICROSCOPY, P657