Large Area, Few-Layer Graphene Films on Arbitrary Substrates by Chemical Vapor Deposition

被引:4877
作者
Reina, Alfonso [2 ]
Jia, Xiaoting [2 ]
Ho, John [1 ]
Nezich, Daniel [3 ]
Son, Hyungbin [1 ]
Bulovic, Vladimir [1 ]
Dresselhaus, Mildred S. [1 ,3 ]
Kong, Jing [1 ]
机构
[1] MIT, Dept Elect Engn & Comp Sci, Cambridge, MA 02139 USA
[2] MIT, Dept Mat Sci & Engn, Cambridge, MA 02139 USA
[3] MIT, Dept Phys, Cambridge, MA 02139 USA
基金
美国国家科学基金会;
关键词
SILVER ATOMS; GRAPHITE; MONOLAYER; NICKEL; PHASE; GAS; ADSORPTION; DEVICES; PT(111);
D O I
10.1021/nl801827v
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
In this work we present a low cost and scalable technique, via ambient pressure chemical vapor deposition (CVD) on polycrystalline Ni films, to fabricate large area (similar to cm(2)) films of single- to few-layer graphene and to transfer the films to nonspecific substrates. These films consist of regions of 1 to similar to 12 graphene layers. Single- or bilayer regions can be up to 20 mu m in lateral size. The films are continuous over the entire area and can be patterned lithographically or by prepatterning the underlying Ni film. The transparency, conductivity, and ambipolar transfer characteristics of the films suggest their potential as another materials candidate for electronics and opto-electronic applications.
引用
收藏
页码:30 / 35
页数:6
相关论文
共 44 条
  • [31] Gate-induced insulating state in bilayer graphene devices
    Oostinga, Jeroen B.
    Heersche, Hubert B.
    Liu, Xinglan
    Morpurgo, Alberto F.
    Vandersypen, Lieven M. K.
    [J]. NATURE MATERIALS, 2008, 7 (02) : 151 - 157
  • [32] REINA A, 2008, J PHYS CHEM C
  • [33] Detection of individual gas molecules adsorbed on graphene
    Schedin, F.
    Geim, A. K.
    Morozov, S. V.
    Hill, E. W.
    Blake, P.
    Katsnelson, M. I.
    Novoselov, K. S.
    [J]. NATURE MATERIALS, 2007, 6 (09) : 652 - 655
  • [34] Synthesis of graphene-based nanosheets via chemical reduction of exfoliated graphite oxide
    Stankovich, Sasha
    Dikin, Dmitriy A.
    Piner, Richard D.
    Kohlhaas, Kevin A.
    Kleinhammes, Alfred
    Jia, Yuanyuan
    Wu, Yue
    Nguyen, SonBinh T.
    Ruoff, Rodney S.
    [J]. CARBON, 2007, 45 (07) : 1558 - 1565
  • [35] Intercalation of silver atoms under a graphite monolayer on Ni(111)
    Starodubov, AG
    Medvetskii, MA
    Shikin, AM
    Adamchuk, VK
    [J]. PHYSICS OF THE SOLID STATE, 2004, 46 (07) : 1340 - 1348
  • [36] Carbon films grown on Pt(111) as supports for model gold catalysts
    Starr, D. E.
    Pazhetnov, E. M.
    Stadnichenko, A. I.
    Boronin, A. I.
    Shaikhutdinov, S. K.
    [J]. SURFACE SCIENCE, 2006, 600 (13) : 2688 - 2695
  • [37] Au-induced encapsulation of Ge nanowires in protective C shells
    Sutter, Eli
    Sutter, Peter
    [J]. ADVANCED MATERIALS, 2006, 18 (19) : 2583 - +
  • [38] Epitaxial graphene on ruthenium
    Sutter, Peter W.
    Flege, Jan-Ingo
    Sutter, Eli A.
    [J]. NATURE MATERIALS, 2008, 7 (05) : 406 - 411
  • [39] Highly oriented monolayer graphite formation on Pt(111) by a supersonic methane beam
    Ueta, H
    Saida, M
    Nakai, C
    Yamada, Y
    Sasaki, M
    Yamamoto, S
    [J]. SURFACE SCIENCE, 2004, 560 (1-3) : 183 - 190
  • [40] The adsorption and decomposition of acetylene on clean and K-covered Co(0001)
    Vaari, J
    Lahtinen, J
    Hautojarvi, P
    [J]. CATALYSIS LETTERS, 1997, 44 (1-2) : 43 - 49