Fabrication of Flexible MoS2 Thin-Film Transistor Arrays for Practical Gas-Sensing Applications

被引:860
作者
He, Qiyuan [1 ]
Zeng, Zhiyuan [1 ]
Yin, Zongyou [1 ]
Li, Hai [1 ]
Wu, Shixin [1 ]
Huang, Xiao [1 ]
Zhang, Hua [1 ]
机构
[1] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore
基金
新加坡国家研究基金会;
关键词
MoS2; reduced graphene oxides; thin-film transistors; gas sensors; flexible electronics; FIELD-EFFECT TRANSISTORS; GRAPHENE OXIDE; CARBON NANOTUBES; CHEMICAL SENSORS; BANDGAP; PHOTOLUMINESCENCE; TRANSPARENT; ENHANCEMENT; NANOWIRES;
D O I
10.1002/smll.201201224
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
By combining two kinds of solution-processable two-dimensional materials, a flexible transistor array is fabricated in which MoS2 thin film is used as the active channel and reduced graphene oxide (rGO) film is used as the drain and source electrodes. The simple device configuration and the 1.5 mm-long MoS2 channel ensure highly reproducible device fabrication and operation. This flexible transistor array can be used as a highly sensitive gas sensor with excellent reproducibility. Compared to using rGO thin film as the active channel, this new gas sensor exhibits much higher sensitivity. Moreover, functionalization of the MoS2 thin film with Pt nanoparticles further increases the sensitivity by up to similar to 3 times. The successful incorporation of a MoS2 thin-film into the electronic sensor promises its potential application in various electronic devices.
引用
收藏
页码:2994 / 2999
页数:6
相关论文
共 65 条
[1]   Carbon nanotube field-effect-transistor-based biosensors [J].
Allen, Brett Lee ;
Kichambare, Padmakar D. ;
Star, Alexander .
ADVANCED MATERIALS, 2007, 19 (11) :1439-1451
[2]  
Balog R, 2010, NAT MATER, V9, P315, DOI [10.1038/nmat2710, 10.1038/NMAT2710]
[3]   Doping graphene by adsorption of polar molecules at the oxidized zigzag edges [J].
Berashevich, Julia ;
Chakraborty, Tapash .
PHYSICAL REVIEW B, 2010, 81 (20)
[4]   Carbon nanotubes based transistors as gas sensors: State of the art and critical review [J].
Bondavalli, Paolo ;
Legagneux, Pierre ;
Pribat, Didier .
SENSORS AND ACTUATORS B-CHEMICAL, 2009, 140 (01) :304-318
[5]   Ultrathin Films of Single-Walled Carbon Nanotubes for Electronics and Sensors: A Review of Fundamental and Applied Aspects [J].
Cao, Qing ;
Rogers, John A. .
ADVANCED MATERIALS, 2009, 21 (01) :29-53
[6]   Preparation of Novel 3D Graphene Networks for Supercapacitor Applications [J].
Cao, Xiehong ;
Shi, Yumeng ;
Shi, Wenhui ;
Lu, Gang ;
Huang, Xiao ;
Yan, Qingyu ;
Zhang, Qichun ;
Zhang, Hua .
SMALL, 2011, 7 (22) :3163-3168
[7]   Optical identification of atomically thin dichalcogenide crystals [J].
Castellanos-Gomez, A. ;
Agrait, N. ;
Rubio-Bollinger, G. .
APPLIED PHYSICS LETTERS, 2010, 96 (21)
[8]   A highly sensitive ultraviolet sensor based on a facile in situ solution-grown ZnO nanorod/graphene heterostructure [J].
Chang, Haixin ;
Sun, Zhenhua ;
Ho, Keith Yat-Fung ;
Tao, Xiaoming ;
Yan, Feng ;
Kwok, Wai-Ming ;
Zheng, Zijian .
NANOSCALE, 2011, 3 (01) :258-264
[9]   Thin Film Field-Effect Phototransistors from Bandgap-Tunable, Solution-Processed, Few-Layer Reduced Graphene Oxide Films [J].
Chang, Haixin ;
Sun, Zhenhua ;
Yuan, Qinghong ;
Ding, Feng ;
Tao, Xiaoming ;
Yan, Feng ;
Zheng, Zijian .
ADVANCED MATERIALS, 2010, 22 (43) :4872-+
[10]   Graphene Field-Effect Transistors: Electrochemical Gating, Interfacial Capacitance, and Biosensing Applications [J].
Chen, Fang ;
Qing, Quan ;
Xia, Jilin ;
Tao, Nongjian .
CHEMISTRY-AN ASIAN JOURNAL, 2010, 5 (10) :2144-2153