Theory of Raman light scattering by nanocrystal acoustic vibrations

被引:27
作者
Gupalov, SV [1 ]
Merkulov, IA [1 ]
机构
[1] Russian Acad Sci, AF Ioffe Physicotech Inst, St Petersburg 194021, Russia
关键词
D O I
10.1134/1.1130997
中图分类号
O469 [凝聚态物理学];
学科分类号
070205 ;
摘要
A theory of Raman scattering of light by acoustic phonons in spherical nanocrystals of zinc-blende and wurtzite semiconductors has been developed with the inclusion of the complex structure of the valence band. The deformation-potential approximation was used to describe the exciton-phonon interaction. It is shown that this approximation allows only Raman scattering processes involving spheroidal acoustic phonons with a total angular momentum F = 0 or 2. The effect of phonon quantum confinement on linewidth in Raman scattering spectra and scattered polarization is analyzed. An expression for the shape of the spectral line corresponding to nonresonant scattering from F=0 phonons was obtained. (C) 1999 American Institute of Physics. [S1063-7834(99)02508-3].
引用
收藏
页码:1349 / 1358
页数:10
相关论文
共 32 条
[1]  
Akhiezer A., 1985, Quantum Electrodynamics
[2]  
Bansal N. P., 1986, HDB GLASS PROPERTIES
[3]  
Berestetskii V B, 1989, QUANTUM ELECTRODYNAM
[4]  
Bir GL., 1974, Symmetry and Strain-Induced Effects in Semiconductors
[5]   FAR-INFRARED AND RAMAN VIBRATIONAL TRANSITIONS OF A SOLID SPHERE - SELECTION-RULES [J].
DUVAL, E .
PHYSICAL REVIEW B, 1992, 46 (09) :5795-5797
[6]   VIBRATION EIGENMODES AND SIZE OF MICROCRYSTALLITES IN GLASS - OBSERVATION BY VERY-LOW-FREQUENCY RAMAN-SCATTERING [J].
DUVAL, E ;
BOUKENTER, A ;
CHAMPAGNON, B .
PHYSICAL REVIEW LETTERS, 1986, 56 (19) :2052-2055
[7]   LUMINESCENCE POLARIZATION OF CDSE MICROCRYSTALS [J].
EFROS, AL .
PHYSICAL REVIEW B, 1992, 46 (12) :7448-7458
[8]  
EFROS AL, 1982, SOV PHYS SEMICOND+, V16, P772
[9]   LOW-FREQUENCY RAMAN-SCATTERING FROM SMALL SILVER PARTICLES EMBEDDED IN SIO2 THIN-FILMS [J].
FUJII, M ;
NAGAREDA, T ;
HAYASHI, S ;
YAMAMOTO, K .
PHYSICAL REVIEW B, 1991, 44 (12) :6243-6248
[10]   Electron-hole long-range exchange interaction in semiconductor quantum dots [J].
Goupalov, SV ;
Ivchenko, EL .
JOURNAL OF CRYSTAL GROWTH, 1998, 184 :393-397