Biomass burning as the main source of organic aerosol particulate matter in Malaysia during haze episodes

被引:118
作者
bin Abas, MR
Oros, DR
Simoneit, BRT [1 ]
机构
[1] Oregon State Univ, Coll Ocean & Atmospher Sci, Environm & Petr Geochem Grp, Corvallis, OR 97331 USA
[2] Univ Malaya, Dept Chem, Kuala Lumpur 50603, Malaysia
关键词
levoglucosan; monosaccharides; sterols; biomass burning;
D O I
10.1016/j.chemosphere.2004.02.002
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
The haze episodes that occurred in Malaysia in September-October 1991, August-October 1994 and September-October 1997 have been attributed to suspended smoke particulate matter from biomass burning in southern Sumatra and Kalimantan, Indonesia. In the present study, polar organic compounds in aerosol particulate matter from Malaysia are converted to their trimethylsilyl derivatives and analyzed by gas chromatography-mass spectrometry in order to better assess the contribution of the biomass burning component during the haze episodes. On the basis of this analysis, levoglucosan was found to be the most abundant organic compound detected in almost all samples. The monosaccharides, alpha- and P-mannose, the lignin breakdown products, vanillic and syringic acids and the minor steroids, cholesterol and P-sitosterol were also present in some samples. The presence of the tracers from smoke overwhelmed the typical signatures of emissions from traffic and other anthropogenic activities in the urban areas. (C) 2004 Elsevier Ltd. All rights reserved.
引用
收藏
页码:1089 / 1095
页数:7
相关论文
共 35 条
[1]  
ABAS MR, 1996, ATMOS ENVIRON, V30, P2779, DOI DOI 10.1016/1352-2310(95)00336-3
[2]  
[Anonymous], 1991, GLOBAL BIOMASS BURNI
[3]   CLIMATE FORCING BY ANTHROPOGENIC AEROSOLS [J].
CHARLSON, RJ ;
SCHWARTZ, SE ;
HALES, JM ;
CESS, RD ;
COAKLEY, JA ;
HANSEN, JE ;
HOFMANN, DJ .
SCIENCE, 1992, 255 (5043) :423-430
[4]   The solvent-extractable organic compounds in the Indonesia biomass burning aerosols - characterization studies [J].
Fang, M ;
Zheng, M ;
Wang, F ;
To, KL ;
Jaafar, AB ;
Tong, SL .
ATMOSPHERIC ENVIRONMENT, 1999, 33 (05) :783-795
[5]   Using levoglucosan as a molecular marker for the long-range transport of biomass combustion aerosols [J].
Fraser, MP ;
Lakshmanan, K .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2000, 34 (21) :4560-4564
[6]   Water-soluble organic compounds in biomass burning aerosols over Amazonia -: 1.: Characterization by NMR and GC-MS -: art. no. 8047 [J].
Graham, B ;
Mayol-Bracero, OL ;
Guyon, P ;
Roberts, GC ;
Decesari, S ;
Facchini, MC ;
Artaxo, P ;
Maenhaut, W ;
Köll, P ;
Andreae, MO .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 2002, 107 (D20) :LBA14-1
[7]   PM-10 HIGH-VOLUME COLLECTION AND QUANTITATION OF SEMIVOLATILE AND NONVOLATILE PHENOLS, METHOXYLATED PHENOLS, ALKANES, AND POLYCYCLIC AROMATIC-HYDROCARBONS FROM WINTER URBAN AIR AND THEIR RELATIONSHIP TO WOOD SMOKE EMISSIONS [J].
HAWTHORNE, SB ;
MILLER, DJ ;
LANGENFELD, JJ ;
KRIEGER, MS .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1992, 26 (11) :2251-2262
[8]  
Levine J. S., 1996, BIOMASS BURNING GLOB, V1
[9]  
Levine JS, 1996, BIOMASS BURNING GLOB, VII
[10]  
Locker H. B., 1988, THESIS DARTMOUTH COL