N-Doped Graphene Natively Grown on Hierarchical Ordered Porous Carbon for Enhanced Oxygen Reduction

被引:399
作者
Liang, Ji [1 ]
Du, Xin [1 ]
Gibson, Christopher [2 ]
Du, Xi Wen [3 ]
Qiao, Shi Zhang [1 ]
机构
[1] Univ Adelaide, Sch Chem Engn, Adelaide, SA 5005, Australia
[2] Flinders Univ S Australia, Sch Chem & Phys Sci, Ctr Nanoscale Sci & Technol, Adelaide, SA 5043, Australia
[3] Tianjin Univ, Sch Mat Sci & Engn, Tianjin 300072, Peoples R China
基金
澳大利亚研究理事会;
关键词
HIGH ELECTROCATALYTIC ACTIVITY; METAL-FREE ELECTROCATALYSTS; NITROGEN; BORON; SUPERCAPACITORS; FRAMEWORKS; CATALYSTS; ELECTRODE; SPHERES; ENERGY;
D O I
10.1002/adma.201302569
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A novel nitrogen-doped hybrid material composed of in situ-formed graphene natively grown on hierarchical ordered porous carbon is prepared, which successfully combines the advantages of both materials, such as high surface area, high mass transfer, and high conductivity. The outstanding structural properties of the resultant material render it an excellent metal-free catalyst for electrochemical oxygen reduction.
引用
收藏
页码:6226 / 6231
页数:6
相关论文
共 36 条
[31]   3D Nitrogen-Doped Graphene Aerogel-Supported Fe3O4 Nanoparticles as Efficient Eletrocatalysts for the Oxygen Reduction Reaction [J].
Wu, Zhong-Shuai ;
Yang, Shubin ;
Sun, Yi ;
Parvez, Khaled ;
Feng, Xinliang ;
Muellen, Klaus .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (22) :9082-9085
[32]   Efficient Metal-Free Oxygen Reduction in Alkaline Medium on High-Surface-Area Mesoporous Nitrogen-Doped Carbons Made from Ionic Liquids and Nucleobases [J].
Yang, Wen ;
Fellinger, Tim-Patrick ;
Antonietti, Markus .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (02) :206-209
[33]   Facile Synthesis of Hierarchically Ordered Porous Carbon via in Situ Self-Assembly of Colloidal Polymer and Silica Spheres and Its Use as a Catalyst Support [J].
Zhang, Shiling ;
Chen, Ling ;
Zhou, Shuxue ;
Zhao, Dongyuan ;
Wu, Limin .
CHEMISTRY OF MATERIALS, 2010, 22 (11) :3433-3440
[34]   Two-Step Boron and Nitrogen Doping in Graphene for Enhanced Synergistic Catalysis [J].
Zheng, Yao ;
Jiao, Yan ;
Ge, Lei ;
Jaroniec, Mietek ;
Qiao, Shi Zhang .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (11) :3110-3116
[35]   Nanoporous Graphitic-C3N4@Carbon Metal-Free Electrocatalysts for Highly Efficient Oxygen Reduction [J].
Zheng, Yao ;
Jiao, Yan ;
Chen, Jun ;
Liu, Jian ;
Liang, Ji ;
Du, Aijun ;
Zhang, Weimin ;
Zhu, Zhonghua ;
Smith, Sean C. ;
Jaroniec, Mietek ;
Lu, Gao Qing ;
Qiao, Shi Zhang .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (50) :20116-20119
[36]   Carbon-Based Supercapacitors Produced by Activation of Graphene [J].
Zhu, Yanwu ;
Murali, Shanthi ;
Stoller, Meryl D. ;
Ganesh, K. J. ;
Cai, Weiwei ;
Ferreira, Paulo J. ;
Pirkle, Adam ;
Wallace, Robert M. ;
Cychosz, Katie A. ;
Thommes, Matthias ;
Su, Dong ;
Stach, Eric A. ;
Ruoff, Rodney S. .
SCIENCE, 2011, 332 (6037) :1537-1541