Nonlinear optical properties of fullerenes

被引:33
作者
Kajzar, F [1 ]
Taliani, C [1 ]
Zamboni, R [1 ]
Rossini, S [1 ]
Danieli, R [1 ]
机构
[1] CNR,IST SPETTROSCOPIA MOLEC,I-40126 BOLOGNA,ITALY
关键词
fullerene; optical properties;
D O I
10.1016/0379-6779(96)80099-3
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Nonlinear optical properties of fullerenes, studied by transverse second-harmonic and wave-dispersed third-harmonic generation, are reviewed and discussed. The origin of second-harmonic generation in C-60, as well as its absence, at the limit of dielectric breakdown in C-70 thin films is also discussed. The observed third-harmonic generation chi((3)) susceptibility dispersion in both lower fullerenes C-60 and C-70 is described in terms of the three-level model. In both molecules the two-photon level is found to lie below the one-photon transition level, in good agreement with theoretical calculations and other experimental determinations.
引用
收藏
页码:257 / 263
页数:7
相关论文
共 36 条
[1]   ORGANIC MOLECULAR SOFT FERROMAGNETISM IN A FULLERENE-C60 [J].
ALLEMAND, PM ;
KHEMANI, KC ;
KOCH, A ;
WUDL, F ;
HOLCZER, K ;
DONOVAN, S ;
GRUNER, G ;
THOMPSON, JD .
SCIENCE, 1991, 253 (5017) :301-303
[2]   LARGE INFRARED NONLINEAR OPTICAL-RESPONSE OF C60 [J].
BLAU, WJ ;
BYRNE, HJ ;
CARDIN, DJ ;
DENNIS, TJ ;
HARE, JP ;
KROTO, HW ;
TAYLOR, R ;
WALTON, DRM .
PHYSICAL REVIEW LETTERS, 1991, 67 (11) :1423-1425
[3]   3RD-ORDER OPTICAL SUSCEPTIBILITY OF GLASSES DETERMINED BY 3RD-HARMONIC GENERATION [J].
BUCHALTER, B ;
MEREDITH, GR .
APPLIED OPTICS, 1982, 21 (17) :3221-3224
[4]  
CHOLLET P, 1991, MOL ENG, V1, P35
[5]   NONRESONANT 3RD-ORDER OPTICAL NONLINEARITY OF ALL-CARBON MOLECULES C-60 [J].
GONG, QH ;
SUN, YX ;
XIA, ZJ ;
ZOU, YH ;
GU, ZN ;
ZHOU, XH ;
DI, Q .
JOURNAL OF APPLIED PHYSICS, 1992, 71 (06) :3025-3026
[6]  
HEBARD AF, 1991, NATURE, V350, P660
[7]   OPTICAL 2ND-HARMONIC AND 3RD-HARMONIC GENERATIONS IN C-60 FILM [J].
HOSHI, H ;
NAKAMURA, N ;
MARUYAMA, Y ;
NAKAGAWA, T ;
SUZUKI, S ;
SHIROMARU, H ;
ACHIBA, Y .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 1991, 30 (8A) :L1397-L1398
[8]   OFF-RESONANT NONLINEAR OPTICAL-PROPERTIES OF C60 STUDIED BY DEGENERATE 4-WAVE-MIXING [J].
KAFAFI, ZH ;
LINDLE, JR ;
PONG, RGS ;
BARTOLI, FJ ;
LINGG, LJ ;
MILLIKEN, J .
CHEMICAL PHYSICS LETTERS, 1992, 188 (5-6) :492-496
[9]   3RD-HARMONIC GENERATION IN LIQUIDS [J].
KAJZAR, F ;
MESSIER, J .
PHYSICAL REVIEW A, 1985, 32 (04) :2352-2363
[10]   WAVE-DISPERSED 3RD-ORDER NONLINEAR-OPTICAL PROPERTIES OF C-60 THIN-FILMS [J].
KAJZAR, F ;
TALIANI, C ;
DANIELI, R ;
ROSSINI, S ;
ZAMBONI, R .
CHEMICAL PHYSICS LETTERS, 1994, 217 (04) :418-422