The need for ammonia abatement with respect to secondary PM reductions in Europe

被引:183
作者
Erisman, JW
Schaap, M
机构
[1] Energy Res Ctr Netherlands, ECN, NL-1755 LE Petten, Netherlands
[2] Univ Utrecht, IMAU, Inst Marine & Atmospher Res, NL-3508 TA Utrecht, Netherlands
关键词
ammonia; abatement; particulate matter; sulphur; nitrogen oxides;
D O I
10.1016/j.envpol.2003.08.042
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
In Europe, secondary particulate matter (PM) comprises 50% or more of PM 2.5. To reduce PM concentrations requires lowering precursor emissions. Since the 1980s, SO2 emissions have decreased by more than 60%, while particle concentrations have decreased less. NOx and NH3 emissions have decreased slightly. The role of ammonia in particle formation is addressed here. It is shown that secondary PM concentrations can only be effectively reduced if ammonia emissions are decreased in much the same way as those Of SO2 and NOx. (C) 2003 Elsevier Ltd. All rights reserved.
引用
收藏
页码:159 / 163
页数:5
相关论文
共 11 条
[1]   Global concentrations of tropospheric sulfate, nitrate, and ammonium aerosol simulated in a general circulation model [J].
Adams, PJ ;
Seinfeld, JH ;
Koch, DM .
JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 1999, 104 (D11) :13791-13823
[2]  
ADAMS PJ, 1999, J GEOPHYS RES, V104, P823
[3]   Response of inorganic PM to precursor concentrations [J].
Ansari, AS ;
Pandis, SN .
ENVIRONMENTAL SCIENCE & TECHNOLOGY, 1998, 32 (18) :2706-2714
[4]   Air pollution and health [J].
Brunekreef, B ;
Holgate, ST .
LANCET, 2002, 360 (9341) :1233-1242
[5]   The European perspective on nitrogen emission and deposition [J].
Erisman, JW ;
Grennfelt, P ;
Sutton, M .
ENVIRONMENT INTERNATIONAL, 2003, 29 (2-3) :311-325
[6]  
González CR, 2003, ATMOS CHEM PHYS, V3, P521
[7]   Effects of atmospheric ammonia (NH3) on terrestrial vegetation:: a review [J].
Krupa, SV .
ENVIRONMENTAL POLLUTION, 2003, 124 (02) :179-221
[8]   ISORROPIA: A new thermodynamic equilibrium model for multiphase multicomponent inorganic aerosols [J].
Nenes, A ;
Pandis, SN ;
Pilinis, C .
AQUATIC GEOCHEMISTRY, 1998, 4 (01) :123-152
[9]   Global air emission inventories for anthropogenic sources of NOx, NH3 and N2O in 1990 [J].
Olivier, JGJ ;
Bouwman, AF ;
Van der Hoek, KW ;
Berdowski, JJM .
ENVIRONMENTAL POLLUTION, 1998, 102 :135-148
[10]   Constructing the European aerosol nitrate concentration field from quality analysed data [J].
Schaap, M ;
Müller, K ;
ten Brink, HM .
ATMOSPHERIC ENVIRONMENT, 2002, 36 (08) :1323-1335