Progress, Challenges, and Opportunities in Two-Dimensional Materials Beyond Graphene

被引:4181
作者
Butler, Sheneve Z. [1 ]
Hollen, Shawna M. [2 ]
Cao, Linyou [3 ]
Cui, Yi [4 ]
Gupta, Jay A. [2 ]
Gutierrez, Humberto R. [14 ]
Heinz, Tony F. [5 ]
Hong, Seung Sae [4 ]
Huang, Jiaxing [6 ]
Ismach, Ariel F. [7 ,8 ]
Johnston-Halperin, Ezekiel [2 ]
Kuno, Masaru [9 ]
Plashnitsa, Vladimir V. [9 ]
Robinson, Richard D. [10 ]
Ruoff, Rodney S. [7 ,8 ]
Salahuddin, Sayeef [11 ]
Shan, Jie [12 ]
Shi, Li
Spencer, Michael G. [13 ]
Terrones, Mauricio [14 ]
Windl, Wolfgang [15 ]
Goldberger, Joshua E. [1 ]
机构
[1] Ohio State Univ, Dept Chem & Biochem, Columbus, OH 43210 USA
[2] Ohio State Univ, Dept Phys, Columbus, OH 43210 USA
[3] N Carolina State Univ, Dept Mat Sci & Engn, Raleigh, NC 27607 USA
[4] Stanford Univ, Dept Mat Sci & Engn, Palo Alto, CA 94305 USA
[5] Columbia Univ, Dept Phys & Elect Engn, New York, NY 10027 USA
[6] Northwestern Univ, Dept Mat Sci & Engn, Evanston, IL 60208 USA
[7] Univ Texas Austin, Dept Mech Engn, Austin, TX 78712 USA
[8] Univ Texas Austin, Mat Sci & Engn Program, Austin, TX 78712 USA
[9] Univ Notre Dame, Dept Chem & Biochem, Notre Dame, IN 46556 USA
[10] Cornell Univ, Dept Mat Sci & Engn, Ithaca, NY 14853 USA
[11] Univ Calif Berkeley, Dept Elect Engn & Comp Sci, Berkeley, CA 94720 USA
[12] Case Western Reserve Univ, Dept Phys, Cleveland, OH 44106 USA
[13] Cornell Univ, Dept Elect & Comp Engn, Ithaca, NY 14850 USA
[14] Penn State Univ, Dept Phys, University Pk, PA 16802 USA
[15] Ohio State Univ, Dept Mat Sci & Engn, Columbus, OH 43210 USA
基金
美国国家科学基金会;
关键词
two-dimensional materials; graphene; nanosheets; graphane; van der Waals epitaxy; van der Waals solid; DER-WAALS EPITAXY; CHEMICAL-VAPOR-DEPOSITION; HEXAGONAL BORON-NITRIDE; TRANSITION-METAL DICHALCOGENIDES; LITHIUM INTERCALATION PROPERTIES; LANGMUIR-BLODGETT DEPOSITION; ENERGY-ELECTRON-DIFFRACTION; HIGH-QUALITY GRAPHENE; MOS2 ATOMIC LAYERS; SINGLE DIRAC CONE;
D O I
10.1021/nn400280c
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Graphene's success has shown that it is possible to create stable, single and few-atom-thick layers of van der Waals materials, and also that these materials can exhibit fascinating and technologically useful properties. Here we review the state-of-the-art of 2D materials beyond graphene. Initially, we will outline the different chemical classes of 2D materials and discuss the various strategies to prepare single-layer, few-layer, and multilayer assembly materials in solution, on substrates, and on the wafer scale. Additionally, we present an experimental guide for identifying and characterizing single-layer-thick materials, as well as outlining emerging techniques that yield both local and global information. We describe the differences that occur in the electronic structure between the bulk and the single layer and discuss various methods of tuning their electronic properties by manipulating the surface. Finally, we highlight the properties and advantages of single-, few-, and many-layer 2D materials in field-effect transistors, spin- and valley-tronics, thermoelectrics, and topological insulators, among many other applications.
引用
收藏
页码:2898 / 2926
页数:29
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