One-pot green synthesis of nitrogen-doped carbon nanoparticles as fluorescent probes for mercury ions

被引:286
作者
Huang, Hong [1 ]
Lv, Jing-Jing [1 ]
Zhou, Dan-Ling [1 ]
Bao, Ning [2 ]
Xu, Yue [1 ]
Wang, Ai-Jun [1 ]
Feng, Jiu-Ju [1 ]
机构
[1] Zhejiang Normal Univ, Coll Chem & Life Sci, Coll Geog & Environm Sci, Jinhua 321004, Peoples R China
[2] Nantong Univ, Sch Publ Hlth, Nantong 226019, Peoples R China
来源
RSC ADVANCES | 2013年 / 3卷 / 44期
关键词
LABEL-FREE DETECTION; GRAPHENE QUANTUM DOTS; ONE-STEP SYNTHESIS; SENSING PLATFORM; HYDROTHERMAL SYNTHESIS; SENSITIVE DETECTION; SELECTIVE DETECTION; HIGHLY EFFICIENT; FACILE SYNTHESIS; NANODOTS;
D O I
10.1039/c3ra43452d
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Herein, a simple, green, and low-cost way was developed in the synthesis of fluorescent nitrogen-doped carbon nanoparticles (FNCPs) with nitrogen content of 6.88%, using one-pot hydrothermal treatment of strawberry juice. The as-prepared FNCPs exhibited a maximum emission at 427 nm with a quantum yield of 6.3%, which could be specifically quenched by Hg2+. This phenomenon was used to develop a fluorescent method for facile detection of Hg2+ with a linear range from 10 nM to 50 mu M and a detection limit of 3 nM (S/N = 3), and further extended to measure environmental water samples with satisfactory recovery. This study provides a green strategy in the synthesis of FNCPs to detect Hg2+ with good performance.
引用
收藏
页码:21691 / 21696
页数:6
相关论文
共 54 条
[1]   Luminescent Carbon Nanodots: Emergent Nanolights [J].
Baker, Sheila N. ;
Baker, Gary A. .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (38) :6726-6744
[2]   Carbon Nanoparticles as Visible-Light Photocatalysts for Efficient CO2 Conversion and Beyond [J].
Cao, Li ;
Sahu, Sushant ;
Anilkumar, Parambath ;
Bunker, Christopher E. ;
Xu, Juan ;
Fernando, K. A. Shiral ;
Wang, Ping ;
Guliants, Elena A. ;
Tackett, Kenneth N., II ;
Sun, Ya-Ping .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (13) :4754-4757
[3]   Interfacing water soluble nanomaterials with fluorescence chemosensing: Graphene quantum dot to detect Hg2+ in 100% aqueous solution [J].
Chakraborti, Himadri ;
Sinha, Sougata ;
Ghosh, Subrata ;
Pal, Suman Kalyan .
MATERIALS LETTERS, 2013, 97 :78-80
[4]   Large scale synthesis of photoluminescent carbon nanodots and their application for bioimaging [J].
Chen, Bisang ;
Li, Feiming ;
Li, Shunxing ;
Weng, Wen ;
Guo, Hongxu ;
Guo, Tao ;
Zhang, Xiaoyang ;
Chen, Yabin ;
Huang, Tingting ;
Hong, Xiaolin ;
You, Shiyu ;
Lin, Yuemei ;
Zeng, Kunhong ;
Chen, Shen .
NANOSCALE, 2013, 5 (05) :1967-1971
[5]   The toxicology of mercury and its chemical compounds [J].
Clarkson, Thomas W. ;
Magos, Laszlo .
CRITICAL REVIEWS IN TOXICOLOGY, 2006, 36 (08) :609-662
[6]   Carbon-Based Dots Co-doped with Nitrogen and Sulfur for High Quantum Yield and Excitation-Independent Emission [J].
Dong, Yongqiang ;
Pang, Hongchang ;
Yang, Hong Bin ;
Guo, Chunxian ;
Shao, Jingwei ;
Chi, Yuwu ;
Li, Chang Ming ;
Yu, Ting .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (30) :7800-7804
[7]   Graphene Quantum Dot as a Green and Facile Sensor for Free Chlorine in Drinking Water [J].
Dong, Yongqiang ;
Li, Geli ;
Zhou, Nana ;
Wang, Ruixue ;
Chi, Yuwu ;
Chen, Guonan .
ANALYTICAL CHEMISTRY, 2012, 84 (19) :8378-8382
[8]   Polyamine-Functionalized Carbon Quantum Dots as Fluorescent Probes for Selective and Sensitive Detection of Copper Ions [J].
Dong, Yongqiang ;
Wang, Ruixue ;
Li, Geli ;
Chen, Congqiang ;
Chi, Yuwu ;
Chen, Guonan .
ANALYTICAL CHEMISTRY, 2012, 84 (14) :6220-6224
[9]   Polyamine-functionalized carbon quantum dots for chemical sensing [J].
Dong, Yongqiang ;
Wang, Ruixue ;
Li, Hao ;
Shao, Jingwei ;
Chi, Yuwu ;
Lin, Xiaomei ;
Chen, Guonan .
CARBON, 2012, 50 (08) :2810-2815
[10]   Extraction of Electrochemiluminescent Oxidized Carbon Quantum Dots from Activated Carbon [J].
Dong, Yongqiang ;
Zhou, Nana ;
Lin, Xiaomei ;
Lin, Jianpeng ;
Chi, Yuwu ;
Chen, Guonan .
CHEMISTRY OF MATERIALS, 2010, 22 (21) :5895-5899