The semiclassical limit of the intermediate scattering function

被引:2
作者
Bonella, S
Ciccotti, G
Coker, DF
机构
[1] UNIV ROMA LA SAPIENZA,DIPARTIMENTO FIS,I-00185 ROME,ITALY
[2] CTR EUROPEEN CALCUL ATOM & MOL,LYON 07,FRANCE
[3] BOSTON UNIV,DEPT CHEM,BOSTON,MA 02215
关键词
D O I
10.1080/002689796173606
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
We point out the existence of an oversimplification in a previously derived semiclassical limit for the intermediate scattering function and present a new derivation of the result. The new formula is similar to the previous one and maintains its symmetry properties (i.e. detailed balance). Unfortunately, our expression also contains a new factor, related to the Maslov index of the trajectories appearing in it, that prevents its numerical implementation.
引用
收藏
页码:1203 / 1207
页数:5
相关论文
共 10 条
[1]  
Arnold V.I., 1991, MATH METHODS CLASSIC
[2]   SEMICLASSICAL PROPAGATION - PHASE INDEXES AND THE INITIAL-VALUE FORMALISM [J].
CAMPOLIETI, G ;
BRUMER, P .
PHYSICAL REVIEW A, 1994, 50 (02) :997-1018
[3]  
Filinov VS, 1996, MOL PHYS, V88, P1517, DOI 10.1080/00268979609484533
[4]  
Filinov VS, 1996, MOL PHYS, V88, P1529, DOI 10.1080/00268979609484534
[5]   CELLULAR-DYNAMICS - A NEW SEMICLASSICAL APPROACH TO TIME-DEPENDENT QUANTUM-MECHANICS [J].
HELLER, EJ .
JOURNAL OF CHEMICAL PHYSICS, 1991, 94 (04) :2723-2729
[6]   INELASTIC NEUTRON-SCATTERING FROM CLASSICAL-SYSTEMS STATIONARY-PHASE APPROXIMATION OF THE SCATTERING LAW [J].
KNELLER, GR .
MOLECULAR PHYSICS, 1994, 83 (01) :63-87
[7]  
Maslov V.P., 1981, Semiclassical Approximation in Quantum Mechanics
[8]   SEMICLASSICAL TIME EVOLUTION WITHOUT ROOT SEARCHES - COMMENT [J].
MILLER, WH .
JOURNAL OF CHEMICAL PHYSICS, 1991, 95 (12) :9428-9430
[9]   TIME-DEPENDENT SEMICLASSICAL SCATTERING THEORY .I. POTENTIAL SCATTERING [J].
PECHUKAS, P .
PHYSICAL REVIEW, 1969, 181 (01) :166-&
[10]  
SCHULMAN LS, 1980, TECHNIQUES APPLICATI